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Cited by 792Electrocatalysts for Energy ConversionCO2 Reduction Techniques and CatalystsCatalytic Processes in Materials Science

Oxygen Evolution Reaction in Alkaline Environment: Material Challenges and Solutions

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Xie, Xiaohong, Du, Lei, Yan, Litao, Park, Sehkyu, Qiu, Yang, Sokolowski, Joshua, Wang, Wei, Shao, Yuyan·2022·Advanced Functional Materials
DOI 10.1002/adfm.202110036
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Abstract

The oxygen evolution reaction (OER) generally exists in electrochemistry‐enabled applications that are coupled with cathodic reactions like hydrogen evolution, carbon dioxide reduction, ammonia synthesis, and electrocatalytic hydrogenation. The OER heavily impacts the overall energy efficiency of these devices because the sluggish OER kinetics result in a huge overpotential, thus, a large amount of efficient catalysts are needed. The benchmark iridium and ruthenium (Ir/Ru)‐based materials (mostly used in acid media) are, however, significantly limited by their scarcity. Non‐precious metal‐based catalysts (NPMCs) have emerged as the most promising alternatives; however, they tend to degrade quickly under the harsh operating conditions of typical OER devices. Another challenge is the unsatisfying performance of OER catalysts when integrated in real‐world devices. Herein, the OER active sites for three mainstream types of NPMCs including non‐precious transition metal oxides/(oxy)hydroxides, metal‐free carbon materials, and hybrid non‐precious metal and carbon composites are reviewed. In addition, possible degradation mechanisms for active sites and mitigation strategies are discussed in detail. This review also provides insights into the gaps between R&D of NPMCs for the OER and their applications in practical devices.

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  • The selection of NaOH as the electrolyte is justified by its established reliability and stability for facilitating HER within alkaline media, with the concentration of 1.5 M serving to mitigate side reactions such as oxygen evolution.

    “The selection of NaOH as the electrolyte is justified by its established reliability and stability for facilitating HER within alkaline media, with the concentration of 1.5 M serving to mitigate side reactions such as oxygen evolution [41].”

    From Dual-function aerogel electrocatalyst enabling efficient hydrogen production and ambient-temperature hydrogen detection (2026) · cites this paper as [41]

    Section 6.1 (Water Electrolysis; page unavailable) supports the general use of alkaline electrolytes in cells with cathodic HER. It gives concentrated KOH—not NaOH—as an example and describes OER at the anode. It does not establish that NaOH is especially reliable or stable for HER, or that 1.5 M NaOH mitigates oxygen evolution. (LLM, conf=0.86)

    Experimental — accuracy not yet measured

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Cited by

Sorted by citations

Authors
Xie, X., Du, L., Yan, L., Park, S., Qiu, Y., Sokolowski, J., Wang, W., & Shao, Y.
Affiliations
  • Pacific Northwest National Laboratory (US)
  • Guangzhou University (CN)
Corresponding author
  • Yan, Litao
  • Wang, Wei
  • Shao, Yuyan
ORCID
Venue
Advanced Functional Materials
Publisher
Wiley
Published
2022-03-13
Volume
32
Issue
21
ISSN
  • 1616-301X (ISSN-L)
  • 1616-3028
DOI
10.1002/adfm.202110036
OpenAlex
W4220678590
Cited by
792
References
5
Citations by year
2026: 208 · 2025: 211 · 2024: 197 · 2023: 127 · 2022: 49
FWCI
26.30
Type
journal article
Language
en
Open access
Licence
Locations
  • Advanced Functional Materials (publishedVersion, cc-by-nc)
  • OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
Funders
  • Pacific Northwest National Laboratory
  • U.S. Department of Energy (DE‐AC05‐76RLO1830)
  • National Natural Science Foundation of China (21805064)
  • Natural Science Foundation of Guangdong Province
Topics
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
  • Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
Keywords
oxygen evolution reaction, alkaline electrocatalysis, non-noble metal catalysts, transition metal oxides, transition metal oxyhydroxides, catalyst degradation mechanisms, overpotential, electrochemical water splitting

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