Porphyrin‐Incorporated 2D D–A Polymers with Over 8.5% Polymer Solar Cell Efficiency
Abstract
A copolymerization strategy is developed to utilize porphyrin as a complementary light-harvesting unit (LHU) in D-A polymers. For polymer solar cells (PSCs), the presence of LHUs increases the short-circuit current density (Jsc ) without sacrificing the open-circuit voltage (Voc ) and fill factor (FF). Up to 8.0% power conversion efficiency (PCE) is delivered by PPor-2:PC71 BM single-junction PSCs. A PCE of 8.6% is achieved when a C-PCBSD cathodic interlayer is introduced.
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This material was ranked as the top electron-donor polymer for OSCs.
“This material was ranked as the top electron-donor polymer for OSCs. 42”
From Recent progress in porphyrin-based materials for organic solar cells (2018) · cites this paper as [42]
The work of Hsu et al. led to a big breakthrough, and an efficiency of 8.6% was obtained using a 2D donor-acceptor copolymer A31.
“The work of Hsu et al. led to a big breakthrough, and an astounding e ffi ciency of 8.6% was obtained using a 2D donor -acceptor copolymer ( A31 , Fig. 6).”
From Recent progress in porphyrin-based materials for organic solar cells (2018) · cites this paper as [42]
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Recent progress in porphyrin-based materials for organic solar cells
Mahmood, A., Hu, J.-Y., Xiao, B., Tang, A., Wang, X., & Zhou, E. (2018) · Journal of Materials Chemistry A · doi:10.1039/c8ta06392c · Cited by 311 · see citing works
Wang, L., Shi, S., Ma, D., Chen, S., Gao, C., Wang, M., Shi, K., Li, Y., Li, X., & Wang, H. (2015) · Macromolecules · doi:10.1021/ma502050b · Cited by 39 · see citing works
Luo, X., Wu, F., Xiao, H., Guo, H., Liu, Y., & Tan, S. (2017) · Synthetic Metals · doi:10.1016/j.synthmet.2016.11.026 · Cited by 10 · see citing works
- Authors
- Chao, Y., Jheng, J., Wu, J., Wu, K., Peng, H., Tsai, M., Wang, C., Hsiao, Y., Wang, C., Lin, C., & Hsu, C.
- Affiliations
- National Yang Ming Chiao Tung University (TW)
- National Chi Nan University (TW)
- Corresponding author
- Wang, Chien‐Lung
- Lin, Ching‐Yao
- Hsu, Chain‐Shu
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2014-06-02
- Volume
- 26
- Issue
- 30
- Pages
- 5205-5210
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2052714328
- Cited by
- 119
- References
- 0
- Citations by year
- 2026: 3 · 2025: 1 · 2024: 2 · 2023: 2 · 2022: 6 · 2021: 5 · 2020: 4 · 2019: 6 · 2018: 10 · 2017: 23 · 2016: 21 · 2015: 30 · 2014: 6
- FWCI
- 14.17
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Advanced Materials (publishedVersion)
- PubMed (publishedVersion)
- Funders
- National Chiao Tung University
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Organic Electronics and Photovoltaics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Organic Light-Emitting Diodes Research
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Silicon and Solar Cell Technologies
- Keywords
- porphyrins, donor-acceptor polymers, two-dimensional polymers, polymer solar cells, copolymerization, short-circuit current density, power conversion efficiency, PC71BM, open-circuit voltage
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