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Nitrogen‐Superdoped 3D Graphene Networks for High‐Performance Supercapacitors
Abstract
An N‐superdoped 3D graphene network structure with an N‐doping level up to 15.8 at% for high‐performance supercapacitor is designed and synthesized, in which the graphene foam with high conductivity acts as skeleton and nested with N‐superdoped reduced graphene oxide arogels. This material shows a highly conductive interconnected 3D porous structure (3.33 S cm−1), large surface area (583 m 2 g−1), low internal resistance (0.4 Ω), good wettability, and a great number of active sites. Because of the multiple synergistic effects of these features, the supercapacitors based on this material show a remarkably excellent electrochemical behavior with a high specific capacitance (of up to 380, 332, and 245 F g−1 in alkaline, acidic, and neutral electrolytes measured in three‐electrode configuration, respectively, 297 F g−1 in alkaline electrolytes measured in two‐electrode configuration), good rate capability, excellent cycling stability (93.5% retention after 4600 cycles), and low internal resistance (0.4 Ω), resulting in high power density with proper high energy density.
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Metal‐Nitrogen‐Doped Carbon Materials as Highly Efficient Catalysts: Progress and Rational Design
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Encapsulated cobalt nanoparticles as a recoverable catalyst for the hydrolysis of sodium borohydride
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Metadata
- Authors
- Zhang, W., Xu, C., Ma, C., Li, G., Wang, Y., Zhang, K., Li, F., Liu, C., Cheng, H., Du, Y., Tang, N., & Ren, W.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2017-07-24
- Volume
- 29
- Issue
- 36
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2738098190
- Cited by
- 310
- References
- 1
- FWCI
- 15.83
- Type
- journal article
- Language
- en
- Open access
- closed
- Funders
- Ministry of Science and Technology of the People's Republic of China (2014CB921102, 2014CB932402, 2016YFA0200101)
- National Natural Science Foundation of China (51572122, 51325205, 51290273, 51521091)
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- Zhang, W., Xu, C., Ma, C., Li, G., Wang, Y., Zhang, K., Li, F., Liu, C., Cheng, H., Du, Y., Tang, N., & Ren, W. (2017). Nitrogen‐Superdoped 3D Graphene Networks for High‐Performance Supercapacitors. Advanced Materials. https://doi.org/10.1002/adma.201701677
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