The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
High‐Voltage Lithium‐Metal Batteries Enabled by Localized High‐Concentration Electrolytes
Abstract
Rechargeable lithium‐metal batteries (LMBs) are regarded as the “holy grail” of energy‐storage systems, but the electrolytes that are highly stable with both a lithium‐metal anode and high‐voltage cathodes still remain a great challenge. Here a novel “localized high‐concentration electrolyte” (HCE; 1.2 m lithium bis(fluorosulfonyl)imide in a mixture of dimethyl carbonate/bis(2,2,2‐trifluoroethyl) ether (1:2 by mol)) is reported that enables dendrite‐free cycling of lithium‐metal anodes with high Coulombic efficiency (99.5%) and excellent capacity retention (>80% after 700 cycles) of Li||LiNi 1/3 Mn 1/3 Co 1/3 O 2 batteries. Unlike the HCEs reported before, the electrolyte reported in this work exhibits low concentration, low cost, low viscosity, improved conductivity, and good wettability that make LMBs closer to practical applications. The fundamental concept of “localized HCEs” developed in this work can also be applied to other battery systems, sensors, supercapacitors, and other electrochemical systems.
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Cites
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Self-citationLi + Solvation and Ionic Transport in Lithium Solvate Ionic Liquids Diluted by Molecular Solvents
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Pathways for practical high-energy long-cycling lithium metal batteries
Liu, J., Bao, Z., Cui, Y., Dufek, E. J., Goodenough, J. B., Khalifah, P., Li, Q., Liaw, B. Y., Liu, P., Manthiram, A., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0338-x · Cited by 3,412
Self-citationA Growing Appreciation for the Role of LiF in the Solid Electrolyte Interphase
Tan, J., Matz, J., Dong, P., Shen, J., & Ye, M. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202100046 · Cited by 1,019
Regulating Interfacial Chemistry in Lithium‐Ion Batteries by a Weakly Solvating Electrolyte**
Yao, Y., Chen, X., Yan, C., Zhang, X., Cai, W., Huang, J., & Zhang, Q. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202011482 · Cited by 855
Tailoring electrolyte solvation for Li metal batteries cycled at ultra-low temperature
Holoubek, J., Liu, H., Wu, Z., Yin, Y., Xing, X., Cai, G., Yu, S., Zhou, H., Pascal, T. A., Chen, Z., et al. (2021) · Nature Energy · doi:10.1038/s41560-021-00783-z · Cited by 851
High-Efficiency Lithium Metal Batteries with Fire-Retardant Electrolytes
Chen, S., Zheng, J., Yu, L., Ren, X., Engelhard, M. H., Niu, C., Lee, H., Xu, W., Xiao, J., Liu, J., et al. (2018) · Joule · doi:10.1016/j.joule.2018.05.002 · Cited by 654
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Metadata
- Authors
- Chen, S., Zheng, J., Mei, D., Han, K. S., Engelhard, M. H., Zhao, W., Xu, W., Liu, J., & Zhang, J.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-03-25
- Volume
- 30
- Issue
- 21
- Pages
- e1706102-e1706102
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2790076382
- Cited by
- 1,328
- References
- 7
- FWCI
- 38.10
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, S., Zheng, J., Mei, D., Han, K. S., Engelhard, M. H., Zhao, W., Xu, W., Liu, J., & Zhang, J. (2018). High‐Voltage Lithium‐Metal Batteries Enabled by Localized High‐Concentration Electrolytes. Advanced Materials. https://doi.org/10.1002/adma.201706102
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