The DOI matches its Crossref record; 46 of the 46 references it cites were found in a registry or an index.
Efficient Hydrogen Evolution Reaction Catalysis in Alkaline Media by All‐in‐One MoS2 with Multifunctional Active Sites
Abstract
MoS 2 becomes an efficient and durable nonprecious‐metal electrocatalyst for the hydrogen evolution reaction (HER) when it contains multifunctional active sites for water splitting derived from 1T‐phase, defects, S vacancies, exposed Mo edges with expanded interlayer spacings. In contrast to previously reported MoS 2‐based catalysts targeting only a single or few of these characteristics, the all‐in‐one MoS 2 catalyst prepared herein features all of the above active site types. During synthesis, the intercalation of in situ generated NH 3 molecules into MoS 2 sheets affords ammoniated MoS 2 (A‐MoS 2) that predominantly comprises 1T‐MoS 2 and exhibits an expanded interlayer spacing. The subsequent reduction of A‐MoS 2 results in the removal of intercalated NH 3 and H 2 S to form an all‐in‐one MoS 2 with multifunctional active sites mentioned above (R‐MoS 2) that exhibits electrocatalytic HER performance in alkaline media superior to those of all previously reported MoS 2‐based electrocatalysts. In particular, a hybrid MoS 2/nickel foam catalyst outperforms commercial Pt/C in the practically meaningful high‐current region (>25 mA cm−2), demonstrating that R‐MoS 2‐based materials can potentially replace Pt catalysts in practical alkaline HER systems.
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Cites
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Cited by
Recent Advances in Electrocatalytic Hydrogen Evolution Using Nanoparticles
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Nanoarchitectonics for Transition‐Metal‐Sulfide‐Based Electrocatalysts for Water Splitting
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Roadmap and Direction toward High-Performance MoS 2 Hydrogen Evolution Catalysts
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Synthesis, stabilization and applications of 2-dimensional 1T metallic MoS 2
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Metadata
- Authors
- Anjum, M. A. R., Jeong, H. Y., Lee, M. H., Shin, H. S., & Lee, J. S.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-03-30
- Volume
- 30
- Issue
- 20
- Pages
- e1707105-e1707105
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2795113778
- Cited by
- 409
- References
- 46
- FWCI
- 10.91
- Type
- journal article
- Language
- en
- Open access
- closed
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