The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
An Armored Mixed Conductor Interphase on a Dendrite‐Free Lithium‐Metal Anode
Abstract
Lithium‐metal electrodes have undergone a comprehensive renaissance to meet the requirements of high‐energy‐density batteries due to their lowest electrode potential and the very high theoretical capacity. Unfortunately, the unstable interface between lithium and nonaqueous electrolyte induces dendritic Li and low Coulombic efficiency during repeated Li plating/stripping, which is one of the huge obstacles toward practical lithium‐metal batteries. Here, a composite mixed ionic/electronic conductor interphase (MCI) is formed on the surface of Li by in situ chemical reactions of a copper‐fluoride‐based solution and Li metal at room temperature. The as‐obtained MCI film acts like the armor of a soldier to protect the Li‐metal anode by its prioritized lithium storage, high ionic conductivity, and high Young's modulus. The armored MCI can effectively suppress Li‐dendrite growth and work effectively in LiNi 0.5 Co 0.2 Mn 0.3 O 2/Li cells. The armored MCI presents fresh insights into the formation and regulation of the stable electrode–electrolyte interface and an effective strategy to protect Li‐metal anodes in working Li‐metal batteries.
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Citations
Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Cited by
Recent Advances in Energy Chemistry between Solid-State Electrolyte and Safe Lithium-Metal Anodes
Cheng, X.-B., Zhao, C.-Z., Yao, Y.-X., Liu, H., & Zhang, Q. (2019) · Chem · doi:10.1016/j.chempr.2018.12.002 · Cited by 874
Self-citationArtificial Interphases for Highly Stable Lithium Metal Anode
Xu, R., Cheng, X.-B., Yan, C., Zhang, X.-Q., Xiao, Y., Zhao, C.-Z., Huang, J.-Q., & Zhang, Q. (2019) · Matter · doi:10.1016/j.matt.2019.05.016 · Cited by 721
Self-citationLiu, W., Liu, P., & Mitlin, D. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202002297 · Cited by 687
Fluorinated hybrid solid-electrolyte-interphase for dendrite-free lithium deposition
Pathak, R., Chen, K., Gurung, A., Reza, K. M., Bahrami, B., Pokharel, J., Baniya, A., He, W., Wu, F., Zhou, Y., et al. (2020) · Nature Communications · doi:10.1038/s41467-019-13774-2 · Cited by 455
Key Aspects of Lithium Metal Anodes for Lithium Metal Batteries
Ghazi, Z. A., Sun, Z., Sun, C., Qi, F., An, B., Li, F., & Cheng, H. (2019) · Small · doi:10.1002/smll.201900687 · Cited by 382
Metadata
- Authors
- Yan, C., Cheng, X., Yao, Y., Shen, X., Li, B., Li, W., Zhang, R., Huang, J., Li, H., & Zhang, Q.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-09-27
- Volume
- 30
- Issue
- 45
- Pages
- e1804461-e1804461
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2893606738
- Cited by
- 427
- References
- 1
- FWCI
- 21.07
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yan, C., Cheng, X., Yao, Y., Shen, X., Li, B., Li, W., Zhang, R., Huang, J., Li, H., & Zhang, Q. (2018). An Armored Mixed Conductor Interphase on a Dendrite‐Free Lithium‐Metal Anode. Advanced Materials. https://doi.org/10.1002/adma.201804461
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