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Perovskite Photovoltaics: The Significant Role of Ligands in Film Formation, Passivation, and Stability
Open accessAbstract
Due to their outstanding optoelectronic properties, metal halide perovskites have been intensively studied in recent years. The latest certificated efficiency of 23.3% recently achieved in perovskite solar cells (PVSCs) enables them to be used as a very promising candidate for next‐generation photovoltaics. The morphology, defect density, and water resistance of perovskite films have an enormous impact on the performance and stability of PVSCs. Ligands, with coordinating capability, have been widely developed to improve the quality and stability of perovskite materials significantly. In the first section of this review, the role of ligands in fabricating perovskite films by different methods (one‐step, two‐step, and postdeposition treatment) is discussed. In the second section, the progress on ligand‐passivated perovskites via post‐treatment, in situ passivation during perovskite formation, and modifying the substrates before perovskite formation is reviewed. In the third section, a discussion of ligand‐stabilized perovskite films from the perspectives of crystal crosslinking, dimensionality engineering, and interfacial modification is presented. Finally, a summary and an outlook are given.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Kim, H.-S., Lee, C.-R., Im, J.-H., Lee, K.-B., Moehl, T., Marchioro, A., Moon, S.-J., Humphry-Baker, R., Yum, J.-H., Moser, J. E., et al. (2012) · Scientific Reports · doi:10.1038/srep00591 · Cited by 8,092
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
Impact of microstructure on local carrier lifetime in perovskite solar cells
de Quilettes, D. W., Vorpahl, S. M., Stranks, S. D., Nagaoka, H., Eperon, G. E., Ziffer, M. E., Snaith, H. J., & Ginger, D. S. (2015) · Science · doi:10.1126/science.aaa5333 · Cited by 2,198
Post-synthetic halide conversion and selective halogen capture in hybrid perovskites
Solis-Ibarra, D., Smith, I. C., & Karunadasa, H. I. (2015) · Chemical Science · doi:10.1039/c5sc01135c · Cited by 127
Cited by
Rationalization of passivation strategies toward high-performance perovskite solar cells
Zhang, Z., Qiao, L., Meng, K., Long, R., Chen, G., & Gao, P. (2023) · Chemical Society Reviews · doi:10.1039/d2cs00217e · Cited by 357
Carbon-based materials for stable, cheaper and large-scale processable perovskite solar cells
Fagiolari, L., & Bella, F. (2019) · Energy & Environmental Science · doi:10.1039/c9ee02115a · Cited by 355
Cao, Q., Li, Y., Zhang, H., Yang, J., Han, J., Xu, T., Wang, S., Wang, Z., Gao, B., Zhao, J., et al. (2021) · Science Advances · doi:10.1126/sciadv.abg0633 · Cited by 322
Self-citationYang, Z., Dou, J., Kou, S., Dang, J., Ji, Y., Yang, G., Wu, W., Kuang, D., & Wang, M. (2020) · Advanced Functional Materials · doi:10.1002/adfm.201910710 · Cited by 258
Metadata
- Authors
- Zhang, H., Nazeeruddin, M. K., & Choy, W. C. H.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2019-01-02
- Volume
- 31
- Issue
- 8
- Pages
- e1805702-e1805702
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2906063838
- Cited by
- 275
- References
- 5
- FWCI
- 16.39
- Type
- journal article
- Language
- en
- Open access
- green
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