The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
A Novel Multinary Intermetallic as an Active Electrocatalyst for Hydrogen Evolution
Open accessAbstract
Electrochemical water splitting offers an attractive approach for hydrogen production. However, the lack of high‐performance cost‐effective electrocatalyst severely hinders its applications. Here, a multinary high‐entropy intermetallic (HEI) that possesses an unusual periodically ordered structure containing multiple non‐noble elements is reported, which can serve as a highly efficient electrocatalyst for hydrogen evolution. This HEI exhibits excellent activities in alkalinity with an overpotential of 88.2 mV at a current density of 10 mA cm−2 and a Tafel slope of 40.1 mV dec−1, which are comparable to those of noble catalysts. Theoretical calculations reveal that the chemical complexity and surprising atomic configurations provide a strong synergistic function to alter the electronic structure. Furthermore, the unique L1 2‐type ordered structure enables a specific site‐isolation effect to further stabilize the H 2 O/H* adsorption/desorption, which dramatically optimizes the energy barrier of hydrogen evolution. Such an HEI strategy uncovers a new paradigm to develop novel electrocatalyst with superior reaction activities.
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Cites
Enhancing Hydrogen Evolution Activity in Water Splitting by Tailoring Li + -Ni(OH) 2 -Pt Interfaces
Subbaraman, R., Tripkovic, D., Strmcnik, D., Chang, K.-C., Uchimura, M., Paulikas, A. P., Stamenkovic, V., & Markovic, N. M. (2011) · Science · doi:10.1126/science.1211934 · Cited by 3,135
Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
Luo, J., Im, J.-H., Mayer, M. T., Schreier, M., Nazeeruddin, M. K., Park, N.-G., Tilley, S. D., Fan, H. J., & Grätzel, M. (2014) · Science · doi:10.1126/science.1258307 · Cited by 2,509
Zhu, Z., Yin, H., He, C., Al‐Mamun, M., Liu, P., Jiang, L., Zhao, Y., Wang, Y., Yang, H., Tang, Z., et al. (2018) · Advanced Materials · doi:10.1002/adma.201801171 · Cited by 228
Self-citationWang, Z., Li, M., Yu, J., Ge, X., Liu, Y., & Wang, W. (2020) · Advanced Materials · doi:10.1002/adma.201906384 · Cited by 138
Cited by
High-entropy energy materials: challenges and new opportunities
Ma, Y., Ma, Y., Wang, Q., Schweidler, S., Botros, M., Fu, T., Hahn, H., Brezesinski, T., & Breitung, B. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00505g · Cited by 963
High-entropy materials for catalysis: A new frontier
Sun, Y., & Dai, S. (2021) · Science Advances · doi:10.1126/sciadv.abg1600 · Cited by 942
Feng, G., Ning, F., Song, J., Shang, H., Zhang, K., Ding, Z., Gao, P., Chu, W., & Xia, D. (2021) · Journal of the American Chemical Society · doi:10.1021/jacs.1c07643 · Cited by 560
High-entropy alloys in electrocatalysis: from fundamentals to applications
Ren, J.-T., Chen, L., Wang, H.-Y., & Yuan, Z.-Y. (2023) · Chemical Society Reviews · doi:10.1039/d3cs00557g · Cited by 551
A high-entropy atomic environment converts inactive to active sites for electrocatalysis
Zhu, H., Sun, S., Hao, J., Zhuang, Z., Zhang, S., Wang, T., Kang, Q., Lu, S., Wang, X., Lai, F., et al. (2023) · Energy & Environmental Science · doi:10.1039/d2ee03185j · Cited by 509
Metadata
- Authors
- Jia, Z., Yang, T., Sun, L., Zhao, Y., Li, W., Luan, J., Lyu, F., Zhang, L., Kruzic, J. J., Kai, J., Huang, J. C., Lu, J., & Liu, C. T.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2020-04-08
- Volume
- 32
- Issue
- 21
- Pages
- e2000385-e2000385
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W3014562495
- Cited by
- 356
- References
- 4
- FWCI
- 9.06
- Type
- journal article
- Language
- en
- Open access
- green
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- Jia, Z., Yang, T., Sun, L., Zhao, Y., Li, W., Luan, J., Lyu, F., Zhang, L., Kruzic, J. J., Kai, J., Huang, J. C., Lu, J., & Liu, C. T. (2020). A Novel Multinary Intermetallic as an Active Electrocatalyst for Hydrogen Evolution. Advanced Materials. https://doi.org/10.1002/adma.202000385
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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