The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Crystalline‐Amorphous Interfaces Coupling of CoSe2/CoP with Optimized d‐Band Center and Boosted Electrocatalytic Hydrogen Evolution
Abstract
Amorphous and heterojunction materials have been widely used in the field of electrocatalytic hydrogen evolution due to their unique physicochemical properties. However, the current used individual strategy still has limited effects. Hence efficient tailoring tactics with synergistic effect are highly desired. Herein, the authors have realized the deep optimization of catalytic activity by a constructing crystalline–amorphous CoSe 2/CoP heterojunction. Benefiting from the strong electronic coupling at the interfaces, the d‐band center of the material moves further down compared to its crystalline–crystalline counterpart, optimizing the valence state and the H adsorption of Co and lowering the kinetic barrier of hydrogen evolution reaction (HER). The heterojunction shows an overpotential of 65 mV to drive a current density of 10 mA cm−2 in the acidic medium. Besides, it also shows competitive properties in both neutral and basic media. This work provides inspiration for optimizing the catalytic activity through combining a crystalline and amorphous heterojunction, which can be implemented for other transition metal compound electrocatalysts.
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Tian, J., Liu, Q., Asiri, A. M., & Sun, X. (2014) · Journal of the American Chemical Society · doi:10.1021/ja503372r · Cited by 2,373
Highly Active Electrocatalysis of the Hydrogen Evolution Reaction by Cobalt Phosphide Nanoparticles
Popczun, E. J., Read, C. G., Roske, C. W., Lewis, N. S., & Schaak, R. E. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201402646 · Cited by 1,240
Jiang, K., Liu, B., Luo, M., Ning, S., Peng, M., Zhao, Y., Lu, Y.-R., Chan, T.-S., de Groot, F. M. F., & Tan, Y. (2019) · Nature Communications · doi:10.1038/s41467-019-09765-y · Cited by 670
Luo, X., Ji, P., Wang, P., Cheng, R., Chen, D., Lin, C., Zhang, J., He, J., Shi, Z., Li, N., et al. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201903891 · Cited by 636
Amorphous nanomaterials in electrocatalytic water splitting
Guo, C., Shi, Y., Lu, S., Yu, Y., & Zhang, B. (2021) · Chinese Journal of Catalysis · doi:10.1016/s1872-2067(20)63740-8 · Cited by 179
Cited by
Gao, G., Zhu, G., Chen, X., Sun, Z., & Cabot, A. (2023) · ACS Nano · doi:10.1021/acsnano.3c05810 · Cited by 278
Liu, Y., Sakthivel, T., Hu, F., Tian, Y., Wu, D., Ang, E. H., Liu, H., Guo, S., Peng, S., & Dai, Z. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202203797 · Cited by 267
Shen, S., Hu, Z., Zhang, H., Song, K., Wang, Z., Lin, Z., Zhang, Q., Gu, L., & Zhong, W. (2022) · Angewandte Chemie International Edition · doi:10.1002/anie.202206460 · Cited by 140
Self-citationXing, M., Zhu, S., Zeng, X., Wang, S., Liu, Z., & Cao, D. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202302376 · Cited by 105
Chen, Y., Li, J., Wang, N., Zhou, Y., Zheng, J., & Chu, W. (2022) · Chemical Engineering Journal · doi:10.1016/j.cej.2022.137611 · Cited by 88
Metadata
- Authors
- Shen, S., Wang, Z., Lin, Z., Song, K., Zhang, Q., Meng, F., Gu, L., & Zhong, W.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2022-02-18
- Volume
- 34
- Issue
- 13
- Pages
- e2110631-e2110631
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W4206027834
- Cited by
- 575
- References
- 5
- FWCI
- 22.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shen, S., Wang, Z., Lin, Z., Song, K., Zhang, Q., Meng, F., Gu, L., & Zhong, W. (2022). Crystalline‐Amorphous Interfaces Coupling of CoSe2/CoP with Optimized d‐Band Center and Boosted Electrocatalytic Hydrogen Evolution. Advanced Materials. https://doi.org/10.1002/adma.202110631
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