The DOI matches its Crossref record; 13 of the 13 references it cites were found in a registry or an index.
Engineering MoS2 Basal Planes for Hydrogen Evolution via Synergistic Ruthenium Doping and Nanocarbon Hybridization
Open accessAbstract
Promoting the intrinsic activity and accessibility of basal plane sites in 2D layered metal dichalcogenides is desirable to optimize their catalytic performance for energy conversion and storage. Herein, a core/shell structured hybrid catalyst, which features few‐layered ruthenium (Ru)‐doped molybdenum disulfide (MoS 2) nanosheets closely sheathing around multiwalled carbon nanotube (CNT), for highly efficient hydrogen evolution reaction (HER) is reported. With 5 at% (atomic percent) Ru substituting for Mo in MoS 2, Ru‐MoS 2/CNT achieves the optimum HER activity, which displays a small overpotential of 50 mV at −10 mA cm−2 and a low Tafel slope of 62 mV dec−1 in 1 m KOH. Theoretical simulations reveal that Ru substituting for Mo in coordination with six S atoms is thermodynamically stable, and the in‐plane S atoms neighboring Ru dopants represent new active centers for facilitating water adsorption, dissociation, and hydrogen adsorption/desorption. This work provides a multiscale structural and electronic engineering strategy for synergistically enhancing the HER activity of transition metal dichalcogenides.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
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Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts
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MoS 2 Nanoparticles Grown on Graphene: An Advanced Catalyst for the Hydrogen Evolution Reaction
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Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution
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MoSe 2 and WSe 2 Nanofilms with Vertically Aligned Molecular Layers on Curved and Rough Surfaces
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Photoelectrochemical water splitting in separate oxygen and hydrogen cells
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Cited by
Recent Advances and Prospective in Ruthenium-Based Materials for Electrochemical Water Splitting
Yu, J., He, Q., Yang, G., Zhou, W., Shao, Z., & Ni, M. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b02457 · Cited by 789
Rational Design of Better Hydrogen Evolution Electrocatalysts for Water Splitting: A Review
Liu, F., Shi, C., Guo, X., He, Z., Pan, L., Huang, Z., Zhang, X., & Zou, J. (2022) · Advanced Science · doi:10.1002/advs.202200307 · Cited by 455
Self-citationRoadmap and Direction toward High-Performance MoS 2 Hydrogen Evolution Catalysts
Cao, Y. (2021) · ACS Nano · doi:10.1021/acsnano.1c01879 · Cited by 405
Zhang, S., Zhang, Z., Si, Y., Li, B., Deng, F., Yang, L., Liu, X., Dai, W., & Luo, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c05834 · Cited by 394
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Metadata
- Authors
- Zhang, X., Zhou, F., Zhang, S., Liang, Y., & Wang, R.
- Venue
- Advanced Science
- Publisher
- Wiley
- Published
- 2019-03-20
- Volume
- 6
- Issue
- 10
- Pages
- 1900090-1900090
- ISSN
- 2198-3844 (ISSN-L)
- OpenAlex
- W2924989184
- Cited by
- 203
- References
- 13
- FWCI
- 6.49
- Type
- journal article
- Language
- en
- Open access
- gold
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- Zhang, X., Zhou, F., Zhang, S., Liang, Y., & Wang, R. (2019). Engineering MoS2 Basal Planes for Hydrogen Evolution via Synergistic Ruthenium Doping and Nanocarbon Hybridization. Advanced Science. https://doi.org/10.1002/advs.201900090
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