The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
An Investigation of Active Sites for electrochemical CO2 Reduction Reactions: From In Situ Characterization to Rational Design
Open accessAbstract
The electrochemical carbon dioxide (CO 2) reduction reaction (CO 2 RR) is among the most promising approaches used to transform greenhouse gas into useful fuels and chemicals. However, the reaction suffers from low selectivity, high overpotential, and low reaction rate. Active site identification in the CO 2 RR is vital for the understanding of the reaction mechanism and the rational development of new electrocatalysts with both high selectivity and stability. Herein, in situ characterization monitoring of active sites during the reaction is summarized and a general understanding of active sites on the various catalysts in the CO 2 RR, including metal‐based catalysts, carbon‐based catalysts, and metal‐organic frameworks‐based electrocatalysts is updated. For each type of electrocatalysts, the reaction pathway and real active sites are proposed based on in situ characterization techniques and theoretical calculations. Finally, the key limitations and challenges observed for the electrochemical fixation of CO 2 is presented. It is expected that this review will provide new insights and directions into further scientific development and practical applicability of CO 2 electroreduction.
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Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
Birdja, Y. Y., Pérez-Gallent, E., Figueiredo, M. C., Göttle, A. J., Calle-Vallejo, F., & Koper, M. T. M. (2019) · Nature Energy · doi:10.1038/s41560-019-0450-y · Cited by 2,747
Hori, Y., Wakebe, H., Tsukamoto, T., & Koga, O. (1994) · Electrochimica Acta · doi:10.1016/0013-4686(94)85172-7 · Cited by 2,140
Dopant-induced electron localization drives CO2 reduction to C2 hydrocarbons
Zhou, Y., Che, F., Liu, M., Zou, C., Liang, Z., De Luna, P., Yuan, H., Li, J., Wang, Z., Xie, H., et al. (2018) · Nature Chemistry · doi:10.1038/s41557-018-0092-x · Cited by 1,171
De Luna, P., Quintero-Bermudez, R., Dinh, C.-T., Ross, M. B., Bushuyev, O. S., Todorović, P., Regier, T., Kelley, S. O., Yang, P., & Sargent, E. H. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0018-9 · Cited by 1,046
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Copper-on-nitride enhances the stable electrosynthesis of multi-carbon products from CO2
Liang, Z.-Q., Zhuang, T.-T., Seifitokaldani, A., Li, J., Huang, C.-W., Tan, C.-S., Li, Y., De Luna, P., Dinh, C. T., Hu, Y., et al. (2018) · Nature Communications · doi:10.1038/s41467-018-06311-0 · Cited by 393
Cited by
Chang, B., Pang, H., Raziq, F., Wang, S., Huang, K.-W., Ye, J., & Zhang, H. (2023) · Energy & Environmental Science · doi:10.1039/d3ee00964e · Cited by 458
Self-citationReview of Carbon Support Coordination Environments for Single Metal Atom Electrocatalysts (SACS)
Song, W., Xiao, C., Ding, J., Huang, Z., Yang, X., Zhang, T., Mitlin, D., & Hu, W. (2024) · Advanced Materials · doi:10.1002/adma.202301477 · Cited by 373
Saleh, H. M., & Hassan, A. I. (2023) · Sustainability · doi:10.3390/su151410891 · Cited by 328
Metadata
- Authors
- Zou, Y., & Wang, S.
- Venue
- Advanced Science
- Publisher
- Wiley
- Published
- 2021-03-03
- Volume
- 8
- Issue
- 9
- Pages
- 2003579-2003579
- ISSN
- 2198-3844 (ISSN-L)
- OpenAlex
- W3134303259
- Cited by
- 189
- References
- 6
- FWCI
- 6.08
- Type
- journal article
- Language
- en
- Open access
- gold
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