The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
SiO2 Hollow Nanosphere‐Based Composite Solid Electrolyte for Lithium Metal Batteries to Suppress Lithium Dendrite Growth and Enhance Cycle Life
Abstract
The low Coulombic efficiency and serious security issues of lithium (Li) metal anode caused by uncontrollable Li dendrite growth have permanently prevented its practical application. A novel SiO 2 hollow nanosphere‐based composite solid electrolyte (SiSE) for Li metal batteries is reported. This hierarchical electrolyte is fabricated via in situ polymerizing the tripropylene gycol diacrylate (TPGDA) monomer in the presence of liquid electrolyte, which is absorbed in a SiO 2 hollow nanosphere layer. The polymerized TPGDA framework keeps the prepared SiSE in a quasi‐solid state without safety risks caused by electrolyte leakage, meanwhile the SiO 2 layer not only acts as a mechanics‐strong separator but also provides the SiSE with high room‐temperature ionic conductivity (1.74 × 10−3 S cm−1) due to the high pore volume (1.49 cm 3 g−1) and large liquid electrolyte uptake of SiO 2 hollow nanospheres. When the SiSE is in situ fabricated on the cathode and applied to LiFePO 4/SiSE/Li batteries, the obtained cells show a significant improvement in cycling stability, mainly attributed to the stable electrode/electrolyte interface and remarkable suppression for Li dendrite growth by the SiSE. This work can extend the application of hollow nanooxide and enable a safe, efficient operation of Li anode in next generation energy storage systems.
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Cites
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Cited by
Polymer Electrolytes for Lithium-Based Batteries: Advances and Prospects
Zhou, D., Shanmukaraj, D., Tkacheva, A., Armand, M., & Wang, G. (2019) · Chem · doi:10.1016/j.chempr.2019.05.009 · Cited by 1,539
Self-citationHighly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries
Fan, X., Chen, L., Ji, X., Deng, T., Hou, S., Chen, J., Zheng, J., Wang, F., Jiang, J., Xu, K., et al. (2018) · Chem · doi:10.1016/j.chempr.2017.10.017 · Cited by 961
Zeng, X.-X., Yin, Y.-X., Li, N.-W., Du, W.-C., Guo, Y.-G., & Wan, L.-J. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b10088 · Cited by 459
High Voltage Operation of Ni‐Rich NMC Cathodes Enabled by Stable Electrode/Electrolyte Interphases
Zhao, W., Zheng, J., Zou, L., Jia, H., Liu, B., Wang, H., Engelhard, M. H., Wang, C., Xu, W., Yang, Y., et al. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201800297 · Cited by 389
Key Aspects of Lithium Metal Anodes for Lithium Metal Batteries
Ghazi, Z. A., Sun, Z., Sun, C., Qi, F., An, B., Li, F., & Cheng, H. (2019) · Small · doi:10.1002/smll.201900687 · Cited by 382
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Metadata
- Authors
- Zhou, D., Liu, R., He, Y., Li, F., Liu, M., Li, B., Yang, Q., Cai, Q., & Kang, F.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2016-01-28
- Volume
- 6
- Issue
- 7
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2291975209
- Cited by
- 408
- References
- 3
- FWCI
- 21.95
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhou, D., Liu, R., He, Y., Li, F., Liu, M., Li, B., Yang, Q., Cai, Q., & Kang, F. (2016). SiO2 Hollow Nanosphere‐Based Composite Solid Electrolyte for Lithium Metal Batteries to Suppress Lithium Dendrite Growth and Enhance Cycle Life. Advanced Energy Materials. https://doi.org/10.1002/aenm.201502214
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