The DOI matches its Crossref record; 50 of the 50 references it cites were found in a registry or an index.
Reshaping Lithium Plating/Stripping Behavior via Bifunctional Polymer Electrolyte for Room-Temperature Solid Li Metal Batteries
Abstract
High-energy rechargeable Li metal batteries are hindered by dendrite growth due to the use of a liquid electrolyte. Solid polymer electrolytes, as promising candidates to solve the above issue, are expected to own high Li ion conductivity without sacrificing mechanical strength, which is still a big challenge to realize. In this study, a bifunctional solid polymer electrolyte exactly having these two merits is proposed with an interpenetrating network of poly(ether–acrylate) (ipn-PEA) and realized via photopolymerization of ion-conductive poly(ethylene oxide) and branched acrylate. The ipn-PEA electrolyte with facile processing capability integrates high mechanical strength (ca. 12 GPa) with high room-temperature ionic conductance (0.22 mS cm –1 ), and significantly promotes uniform Li plating/stripping. Li metal full cells assembled with ipn-PEA electrolyte and cathodes within 4.5 V vs Li + /Li operate effectively at a rate of 5 C and cycle stably at a rate of 1 C at room temperature. Because of its fabrication simplicity and compelling characteristics, the bifunctional ipn-PEA electrolyte reshapes the feasibility of room-temperature solid-state Li metal batteries.
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Cites
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Cited by
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Metadata
- Authors
- Zeng, X.-X., Yin, Y.-X., Li, N.-W., Du, W.-C., Guo, Y.-G., & Wan, L.-J.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-12-06
- Volume
- 138
- Issue
- 49
- Pages
- 15825-15828
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2559131443
- Cited by
- 459
- References
- 50
- FWCI
- 28.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zeng, X.-X., Yin, Y.-X., Li, N.-W., Du, W.-C., Guo, Y.-G., & Wan, L.-J. (2016). Reshaping Lithium Plating/Stripping Behavior via Bifunctional Polymer Electrolyte for Room-Temperature Solid Li Metal Batteries. Journal of the American Chemical Society. https://doi.org/10.1021/jacs.6b10088
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