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Narrowing the Gap between Theoretical and Practical Capacities in Li‐Ion Layered Oxide Cathode Materials
Open accessAbstract
Although layered lithium oxides have become the cathode of choice for state‐of‐the‐art Li‐ion batteries, substantial gaps remain between the practical and theoretical energy densities. With the aim of supporting efforts to close this gap, this work reviews the fundamental operating mechanisms and challenges of Li intercalation in layered oxides, contrasts how these challenges play out differently for different materials (with emphasis on Ni–Co–Al (NCA) and Ni–Mn–Co (NMC) alloys), and summarizes the extensive corpus of modifications and extensions to the layered lithium oxides. Particular emphasis is given to the fundamental mechanisms behind the operation and degradation of layered intercalation electrode materials as well as novel modifications and extensions, including Na‐ion and cation‐disordered materials.
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Cited by
Tsai, P.-C., Wen, B., Wolfman, M., Choe, M.-J., Pan, M. S., Su, L., Thornton, K., Cabana, J., & Chiang, Y.-M. (2018) · Energy & Environmental Science · doi:10.1039/c8ee00001h · Cited by 325
Chakraborty, A., Kunnikuruvan, S., Kumar, S., Markovsky, B., Aurbach, D., Dixit, M., & Major, D. T. (2020) · Chemistry of Materials · doi:10.1021/acs.chemmater.9b04066 · Cited by 322
Kim, T., Ono, L. K., & Qi, Y. (2023) · Journal of Materials Chemistry A · doi:10.1039/d2ta07565b · Cited by 119
Metadata
- Authors
- Radin, M. D., Hy, S., Sina, M., Fang, C., Liu, H., Vinckeviciute, J., Zhang, M., Whittingham, M. S., Meng, Y. S., & Van der Ven, A.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2017-07-04
- Volume
- 7
- Issue
- 20
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2727670264
- Cited by
- 677
- References
- 8
- FWCI
- 21.70
- Type
- journal article
- Language
- en
- Open access
- green
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- Radin, M. D., Hy, S., Sina, M., Fang, C., Liu, H., Vinckeviciute, J., Zhang, M., Whittingham, M. S., Meng, Y. S., & Van der Ven, A. (2017). Narrowing the Gap between Theoretical and Practical Capacities in Li‐Ion Layered Oxide Cathode Materials. Advanced Energy Materials. https://doi.org/10.1002/aenm.201602888
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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