The DOI matches its Crossref record; 54 of the 54 references it cites were found in a registry or an index.
Tunable and Efficient Tin Modified Nitrogen‐Doped Carbon Nanofibers for Electrochemical Reduction of Aqueous Carbon Dioxide
Abstract
Efficient and selective earth‐abundant catalysts are highly desirable to drive the electrochemical conversion of CO 2 into value‐added chemicals. In this work, a low‐cost Sn modified N‐doped carbon nanofiber hybrid catalyst is developed for switchable CO 2 electroreduction in aqueous medium via a straightforward electrospinning technique coupled with a pyrolysis process. The electrocatalytic performance can be tuned by the structure of Sn species on the N‐doped carbon nanofibers. Sn nanoparticles drive efficient formate formation with a high current density of 11 mA cm−2 and a faradaic efficiency of 62% at a moderate overpotential of 690 mV. Atomically dispersed Sn species promote conversion of CO 2 to CO with a high faradaic efficiency of 91% at a low overpotential of 490 mV. The interaction between Sn species and pyridinic‐N may play an important role in tuning the catalytic activity and selectivity of these two materials.
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
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Electrocatalytic carbon dioxide reduction: from fundamental principles to catalyst design
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Metadata
- Authors
- Zhao, Y., Liang, J., Wang, C., Ma, J., & Wallace, G. G.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2018-01-05
- Volume
- 8
- Issue
- 10
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2782656943
- Cited by
- 283
- References
- 54
- FWCI
- 8.99
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhao, Y., Liang, J., Wang, C., Ma, J., & Wallace, G. G. (2018). Tunable and Efficient Tin Modified Nitrogen‐Doped Carbon Nanofibers for Electrochemical Reduction of Aqueous Carbon Dioxide. Advanced Energy Materials. https://doi.org/10.1002/aenm.201702524
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