The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Interpenetrating Triphase Cobalt‐Based Nanocomposites as Efficient Bifunctional Oxygen Electrocatalysts for Long‐Lasting Rechargeable Zn–Air Batteries
Open accessAbstract
Rational construction of atomic‐scale interfaces in multiphase nanocomposites is an intriguing and challenging approach to developing advanced catalysts for both oxygen reduction (ORR) and evolution reactions (OER). Herein, a hybrid of interpenetrating metallic Co and spinel Co 3 O 4 “Janus” nanoparticles stitched in porous graphitized shells (Co/Co 3 O 4@PGS) is synthesized via ionic exchange and redox between Co 2+ and 2D metal–organic‐framework nanosheets. This strategy is proven to effectively establish highways for the transfer of electrons and reactants within the hybrid through interfacial engineering. Specifically, the phase interpenetration of mixed Co species and encapsulating porous graphitized shells provides an optimal charge/mass transport environment. Furthermore, the defect‐rich interfaces act as atomic‐traps to achieve exceptional adsorption capability for oxygen reactants. Finally, robust coupling between Co and N through intimate covalent bonds prohibits the detachment of nanoparticles. As a result, Co/Co 3 O 4@PGS outperforms state‐of‐the‐art noble‐metal catalysts with a positive half‐wave potential of 0.89 V for ORR and a low potential of 1.58 V at 10 mA cm−2 for OER. In a practical demonstration, ultrastable cyclability with a record lifetime of over 800 h at 10 mA cm−2 is achieved by Zn–air batteries with Co/Co 3 O 4@PGS within the rechargeable air electrode.
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Wang, H., Maiyalagan, T., & Wang, X. (2012) · ACS Catalysis · doi:10.1021/cs200652y · Cited by 3,618
Jiang, J., Li, Y., Liu, J., Huang, X., Yuan, C., & Lou, X. W. (. (2012) · Advanced Materials · doi:10.1002/adma.201202146 · Cited by 2,473
Hou, Y., Qiu, M., Nam, G., Kim, M. G., Zhang, T., Liu, K., Zhuang, X., Cho, J., Yuan, C., & Feng, X. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b01030 · Cited by 284
Qian, Y., Liu, Z., Zhang, H., Wu, P., & Cai, C. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b11927 · Cited by 150
Cited by
Zhao, C., Liu, J., Li, B., Ren, D., Chen, X., Yu, J., & Zhang, Q. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202003619 · Cited by 641
Or, T., Gourley, S. W. D., Kaliyappan, K., Yu, A., & Chen, Z. (2020) · Carbon Energy · doi:10.1002/cey2.29 · Cited by 559
Self-citationJin, S., Mu, D., Lu, Z., Li, R., Liu, Z., Wang, Y., Tian, S., & Dai, C. (2022) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2022.130535 · Cited by 361
A Review of Rechargeable Zinc–Air Batteries: Recent Progress and Future Perspectives
Nazir, G., Rehman, A., Lee, J.-H., Kim, C.-H., Gautam, J., Heo, K., Hussain, S., Ikram, M., AlObaid, A. A., Lee, S.-Y., et al. (2024) · Nano-Micro Letters · doi:10.1007/s40820-024-01328-1 · Cited by 328
Wang, X., Yu, M., & Feng, X. (2023) · eScience · doi:10.1016/j.esci.2023.100141 · Cited by 284
Metadata
- Authors
- Jiang, Y., Deng, Y., Fu, J., Lee, D. U., Liang, R., Cano, Z. P., Liu, Y., Bai, Z., Hwang, S., Yang, L., Su, D., Chu, W., & Chen, Z.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2018-01-31
- Volume
- 8
- Issue
- 15
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2790847806
- Cited by
- 326
- References
- 4
- FWCI
- 10.63
- Type
- journal article
- Language
- en
- Open access
- green
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- Jiang, Y., Deng, Y., Fu, J., Lee, D. U., Liang, R., Cano, Z. P., Liu, Y., Bai, Z., Hwang, S., Yang, L., Su, D., Chu, W., & Chen, Z. (2018). Interpenetrating Triphase Cobalt‐Based Nanocomposites as Efficient Bifunctional Oxygen Electrocatalysts for Long‐Lasting Rechargeable Zn–Air Batteries. Advanced Energy Materials. https://doi.org/10.1002/aenm.201702900
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