Cited by 2,473Advancements in Battery MaterialsSupercapacitor Materials and FabricationMXene and MAX Phase Materials

Recent advances in metal oxide-based electrode architecture design for electrochemical energy storage

Jiang, Jian, Li, Yuanyuan, Liu, Jinping, Huang, Xintang, Yuan, Changzhou, Lou, Xiong Wen (David)·2012·Advanced Materials

Abstract

Metal oxide nanostructures are promising electrode materials for lithium-ion batteries and supercapacitors because of their high specific capacity/capacitance, typically 2-3 times higher than that of the carbon/graphite-based materials. However, their cycling stability and rate performance still can not meet the requirements of practical applications. It is therefore urgent to improve their overall device performance, which depends on not only the development of advanced electrode materials but also in a large part "how to design superior electrode architectures". In the article, we will review recent advances in strategies for advanced metal oxide-based hybrid nanostructure design, with the focus on the binder-free film/array electrodes. These binder-free electrodes, with the integration of unique merits of each component, can provide larger electrochemically active surface area, faster electron transport and superior ion diffusion, thus leading to substantially improved cycling and rate performance. Several recently emerged concepts of using ordered nanostructure arrays, synergetic core-shell structures, nanostructured current collectors, and flexible paper/textile electrodes will be highlighted, pointing out advantages and challenges where appropriate. Some future electrode design trends and directions are also discussed.

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Crossref · 10.1002/adma.201202146

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  • Lithium-ion batteries have dominated daily life because of their desirable electrochemical performance in energy density and power density, as well as advances in their system design and manufacturing.

    “Lithium-ion batteries have already dominated our daily life because of their desirable electrochemical performance in both energy density and power density, as well as the advances in their system design and manufacturing.98,99”

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Authors
Jiang, J., Li, Y., Liu, J., Huang, X., Yuan, C., & Lou, X. W. (.
Affiliations
  • Central China Normal University (CN)
  • Huazhong University of Science and Technology (CN)
  • Nanyang Technological University (SG)
Corresponding author
  • Liu, Jinping
  • Lou, Xiong Wen (David)
Venue
Advanced Materials
Publisher
Wiley
Published
2012-08-21
Volume
24
Issue
38
Pages
5166-5180
ISSN
  • 0935-9648 (ISSN-L)
  • 1521-4095
OpenAlex
W2081738501
Cited by
2,473
References
130
Citations by year
2026: 58 · 2025: 70 · 2024: 97 · 2023: 112 · 2022: 108 · 2021: 118 · 2020: 181 · 2019: 208 · 2018: 277 · 2017: 240 · 2016: 305 · 2015: 301 · 2014: 250 · 2013: 135 · 2012: 13
FWCI
13.15
Type
journal article
Language
en
Open access
closed
Locations
  • Advanced Materials (publishedVersion)
  • PubMed (publishedVersion)
  • DR-NTU (Nanyang Technological University) (submittedVersion)
Funders
  • National Natural Science Foundation of China
  • Ministry of Earth Sciences
  • Huazhong University of Science and Technology
  • Natural Science Foundation of Hubei Province
  • Ministry of Education, India
  • Central China Normal University
Topics
  • Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
  • Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
  • Physical Sciences › Materials Science › Materials Chemistry › MXene and MAX Phase Materials
Keywords
metal oxide electrodes, binder-free electrodes, hybrid nanostructures, lithium-ion batteries, supercapacitors, nanostructure arrays, core-shell structure, textile electrodes, cycling stability, rate capability, ion diffusion
MeSH terms
Electrodes, Graphite, Metals, Oxides, Polymers, Electric Power Supplies, Nanostructures, Electrochemical Techniques

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