The DOI matches its Crossref record; 11 of the 11 references it cites were found in a registry or an index.
Carbon‐Tailored Semimetal MoP as an Efficient Hydrogen Evolution Electrocatalyst in Both Alkaline and Acid Media
Open accessAbstract
The electrolysis processes such as hydrogen evolution reaction (HER) require high efficient catalysts with robust surface stability. A high conductivity is also necessary to speed up the charge transport between the catalyst and the electrolyte. Recently, the observation of exceedingly high conductivity in the topological semimetal MoP, has provided a model catalyst to investigate the correlation between the electrical transport and the electrocatalytic activity for the HER. Thus, MoP is encapsulated in a Mo, P codoped carbon layer (MoP@C). This composite material exhibits outstanding HER performance, with an extremely low overpotential of 49 mV at a current density of 10 mA cm−2 and a Tafel slope of 54 mV dec−1 in an alkaline medium. In addition, electron transport analysis indicates that MoP exhibits high conductivity and mobility due to the existence of triple‐point fermions and a complex Fermi surface. Furthermore, the presence of PC and MoC bonds at the interface between the carbon layer and the MoP particles modulates the band structure of MoP@C and facilitates fast electron transfer, accumulation, and subsequent delocalization, which are in turn responsible for the excellent HER activity.
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Cites
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Strategies for design of electrocatalysts for hydrogen evolution under alkaline conditions
Wang, X., Zheng, Y., Sheng, W., Xu, Z. J., Jaroniec, M., & Qiao, S.-Z. (2020) · Materials Today · doi:10.1016/j.mattod.2019.12.003 · Cited by 533
Huang, Y., Hu, L., Liu, R., Hu, Y., Xiong, T., Qiu, W., Balogun, M.-S. (. T., Pan, A., & Tong, Y. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.03.037 · Cited by 336
Rational Design of Transition Metal Phosphide‐Based Electrocatalysts for Hydrogen Evolution
Liu, D., Xu, G., Yang, H., Wang, H., & Xia, B. Y. (2023) · Advanced Functional Materials · doi:10.1002/adfm.202208358 · Cited by 302
Engineering Ni2P-NiSe2 heterostructure interface for highly efficient alkaline hydrogen evolution
Liu, C., Gong, T., Zhang, J., Zheng, X., Mao, J., Liu, H., Li, Y., & Hao, Q. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.118245 · Cited by 278
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Metadata
- Authors
- Li, G., Sun, Y., Rao, J., Wu, J., Kumar, A., Xu, Q. N., Fu, C., Liu, E., Blake, G. R., Werner, P., Shao, B., Liu, K., Parkin, S., Liu, X., Fahlman, M., Liou, S., Auffermann, G., Zhang, J., Felser, C., & Feng, X.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2018-06-25
- Volume
- 8
- Issue
- 24
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2809814889
- Cited by
- 169
- References
- 11
- FWCI
- 4.75
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Li, G., Sun, Y., Rao, J., Wu, J., Kumar, A., Xu, Q. N., Fu, C., Liu, E., Blake, G. R., Werner, P., Shao, B., Liu, K., Parkin, S., Liu, X., Fahlman, M., Liou, S., Auffermann, G., Zhang, J., Felser, C., & Feng, X. (2018). Carbon‐Tailored Semimetal MoP as an Efficient Hydrogen Evolution Electrocatalyst in Both Alkaline and Acid Media. Advanced Energy Materials. https://doi.org/10.1002/aenm.201801258
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