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Modulating Electronic Structure of Metal‐Organic Framework for Efficient Electrocatalytic Oxygen Evolution
Abstract
Exploring effective electrocatalysts for oxygen evolution reaction (OER) is a crucial requirement of many energy storage and conversion systems, involving fuel cells, water splitting, and metal–air batteries. Herein, a heterogeneity metal‐organic framework (MOF) is prepared by the assembling of metals, terephthalic (A) and 2‐aminoterephthalic ligands (B), defined as A 2.7 B‐MOF‐FeCo 1.6. More importantly, A 2.7 B‐MOF‐FeCo 1.6 exhibits excellent OER activity with an ultralow overpotential of 288 mV at 10 mA cm−2 and a Tafel slope of 39 mV dec−1. The high electrocatalytic performance for OER is attributed to the optimized electronic structure of the intrinsic catalytic center in MOFs via the engineering of the metal node and linkers. The work offers not only a benchmark for pure MOFs in electrocatalysis but also a new efficient strategy to improve electrocatalytic performance by electronic structure engineering of catalytic active centers in MOFs.
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Opportunities and challenges for a sustainable energy future
Chu, S., & Majumdar, A. (2012) · Nature · doi:10.1038/nature11475 · Cited by 12,550
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Earth-abundant catalysts for electrochemical and photoelectrochemical water splitting
Roger, I., Shipman, M. A., & Symes, M. D. (2017) · Nature Reviews Chemistry · doi:10.1038/s41570-016-0003 · Cited by 3,503
Anantharaj, S., Ede, S. R., Sakthikumar, K., Karthick, K., Mishra, S., & Kundu, S. (2016) · ACS Catalysis · doi:10.1021/acscatal.6b02479 · Cited by 2,503
Carbon-based electrocatalysts for advanced energy conversion and storage
Zhang, J., Xia, Z., & Dai, L. (2015) · Science Advances · doi:10.1126/sciadv.1500564 · Cited by 735
Yang, Y., Lin, Z., Gao, S., Su, J., Lun, Z., Xia, G., Chen, J., Zhang, R., & Chen, Q. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b02573 · Cited by 423
Cited by
Wu, Y., Li, Y., Gao, J., & Zhang, Q. (2021) · SusMat · doi:10.1002/sus2.3 · Cited by 319
Self-citationJamesh, M.-I., & Harb, M. (2021) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2020.08.001 · Cited by 274
Metadata
- Authors
- Xue, Z., Li, Y., Zhang, Y., Geng, W., Jia, B., Tang, J., Bao, S., Wang, H., Fan, Y., Wei, Z., Zhang, Z., Ke, Z., Li, G., & Su, C.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2018-09-02
- Volume
- 8
- Issue
- 29
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2890079715
- Cited by
- 309
- References
- 7
- FWCI
- 8.88
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xue, Z., Li, Y., Zhang, Y., Geng, W., Jia, B., Tang, J., Bao, S., Wang, H., Fan, Y., Wei, Z., Zhang, Z., Ke, Z., Li, G., & Su, C. (2018). Modulating Electronic Structure of Metal‐Organic Framework for Efficient Electrocatalytic Oxygen Evolution. Advanced Energy Materials. https://doi.org/10.1002/aenm.201801564
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