The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Efficient Visible‐Light‐Driven Carbon Dioxide Reduction by a Single‐Atom Implanted Metal–Organic Framework
Abstract
Modular optimization of metal–organic frameworks (MOFs) was realized by incorporation of coordinatively unsaturated single atoms in a MOF matrix. The newly developed MOF can selectively capture and photoreduce CO 2 with high efficiency under visible‐light irradiation. Mechanistic investigation reveals that the presence of single Co atoms in the MOF can greatly boost the electron–hole separation efficiency in porphyrin units. Directional migration of photogenerated excitons from porphyrin to catalytic Co centers was witnessed, thereby achieving supply of long‐lived electrons for the reduction of CO 2 molecules adsorbed on Co centers. As a direct result, porphyrin MOF comprising atomically dispersed catalytic centers exhibits significantly enhanced photocatalytic conversion of CO 2, which is equivalent to a 3.13‐fold improvement in CO evolution rate (200.6 μmol g−1 h−1) and a 5.93‐fold enhancement in CH 4 generation rate (36.67 μmol g−1 h−1) compared to the parent MOF.
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Cites
Atomic cobalt on nitrogen-doped graphene for hydrogen generation
Fei, H., Dong, J., Arellano-Jiménez, M. J., Ye, G., Dong Kim, N., Samuel, E. L. G., Peng, Z., Zhu, Z., Qin, F., Bao, J., et al. (2015) · Nature Communications · doi:10.1038/ncomms9668 · Cited by 1,621
Self-citationXu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
Cited by
Zhang, L., Han, L., Liu, H., Liu, X., & Luo, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201706921 · Cited by 532
Vu, N., Kaliaguine, S., & Do, T. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201901825 · Cited by 445
Recent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
Ultrasmall MoOx Clusters as a Novel Cocatalyst for Photocatalytic Hydrogen Evolution
Zhang, H., Zhang, P., Qiu, M., Dong, J., Zhang, Y., & Lou, X. W. (. (2019) · Advanced Materials · doi:10.1002/adma.201804883 · Cited by 309
Self-citationXu, G., Zhang, H., Wei, J., Zhang, H.-X., Wu, X., Li, Y., Li, C., Zhang, J., & Ye, J. (2018) · ACS Nano · doi:10.1021/acsnano.8b00110 · Cited by 298
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Metadata
- Authors
- Zhang, H., Wei, J., Dong, J., Liu, G., Shi, L., An, P., Zhao, G., Kong, J., Wang, X., Meng, X., Zhang, J., & Ye, J.
- Venue
- Angewandte Chemie
- Publisher
- Wiley
- Published
- 2016-10-13
- Volume
- 128
- Issue
- 46
- Pages
- 14522-14526
- ISSN
- 0044-8249 (ISSN-L)
- 1521-3757
- OpenAlex
- W4239692985
- Cited by
- 214
- References
- 2
- FWCI
- 5.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, H., Wei, J., Dong, J., Liu, G., Shi, L., An, P., Zhao, G., Kong, J., Wang, X., Meng, X., Zhang, J., & Ye, J. (2016). Efficient Visible‐Light‐Driven Carbon Dioxide Reduction by a Single‐Atom Implanted Metal–Organic Framework. Angewandte Chemie. https://doi.org/10.1002/ange.201608597
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