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Charge Separation in Excited States of Decoupled Systems—TICT Compounds and Implications Regarding the Development of New Laser Dyes and the Primary Process of Vision and Photosynthesis
Abstract
The understanding of the dual fluorescence of certain aromatic systems has greatly advanced in recent years. The accompanying large charge separation has been shown to be linked to a twisted (or small overlap) arrangement of the chromophores. Recent theoretical models are able to describe the excited‐state twisting of both single bonds (TICT compounds) and double bonds (olefins) in a unified picture. These models can help to elucidate the photophysical behavior of many organic, inorganic, and biologically relevant compounds, and their application to laser dyes and fluorescent probes provides a route to new “tailor‐made” fluorescent materials. Applied to the primary processes of vision and photosynthesis, these models can lead to a deeper understanding of basic photobiological processes.
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Cited by
Grabowski, Z. R., Rotkiewicz, K., & Rettig, W. (2003) · Chemical Reviews · doi:10.1021/cr940745l · Cited by 3,714
Self-citationDesign principles of fluorescent molecular sensors for cation recognition
Valeur, B. (2000) · Coordination Chemistry Reviews · doi:10.1016/s0010-8545(00)00246-0 · Cited by 2,377
Spectroscopic studies of nile red in organic solvents and polymers
Dutta, A. K., Kamada, K., & Ohta, K. (1996) · Journal of Photochemistry and Photobiology A: Chemistry · doi:10.1016/1010-6030(95)04140-0 · Cited by 300
Zhang, Q., Yu, P., Fan, Y., Sun, C., He, H., Liu, X., Lu, L., Zhao, M., Zhang, H., & Zhang, F. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202012427 · Cited by 216
Xu, B., Zhang, J., Fang, H., Ma, S., Chen, Q., Sun, H., Im, C., & Tian, W. (2014) · Polym. Chem. · doi:10.1039/c3py00974b · Cited by 56
Metadata
- Authors
- Rettig, W.
- Venue
- Angewandte Chemie International Edition in English
- Publisher
- Wiley
- Published
- 1986-11
- Volume
- 25
- Issue
- 11
- Pages
- 971-988
- ISSN
- 0570-0833 (ISSN-L)
- OpenAlex
- W2110324274
- Cited by
- 1,324
- References
- 0
- FWCI
- 15.95
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rettig, W. (1986). Charge Separation in Excited States of Decoupled Systems—TICT Compounds and Implications Regarding the Development of New Laser Dyes and the Primary Process of Vision and Photosynthesis. Angewandte Chemie International Edition in English. https://doi.org/10.1002/anie.198609711
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