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Gas‐Phase Catalysis by Atomic and Cluster Metal Ions: The Ultimate Single‐Site Catalysts
Abstract
Gas‐phase experiments with state‐of‐the‐art techniques of mass spectrometry provide detailed insights into numerous elementary processes. The focus of this Review is on elementary reactions of ions that achieve complete catalytic cycles under thermal conditions. The examples chosen cover aspects of catalysis pertinent to areas as diverse as atmospheric chemistry and surface chemistry. We describe how transfer of oxygen atoms, bond activation, and coupling of fragments can be mediated by atomic or cluster metal ions. In some cases truly unexpected analogies of the idealized gas‐phase ion catalysis can be drawn with related chemical transformations in solution or the solid state, and so improve our understanding of the intrinsic operation of a practical catalyst at a strictly molecular level.
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Citations
Cites
Charging Effects on Bonding and Catalyzed Oxidation of CO on Au 8 Clusters on MgO
Yoon, B., Häkkinen, H., Landman, U., Wörz, A. S., Antonietti, J.-M., Abbet, S., Judai, K., & Heiz, U. (2005) · Science · doi:10.1126/science.1104168 · Cited by 1,430
Cited by
Single-atom catalysis of CO oxidation using Pt1/FeOx
Qiao, B., Wang, A., Yang, X., Allard, L. F., Jiang, Z., Cui, Y., Liu, J., Li, J., & Zhang, T. (2011) · Nature Chemistry · doi:10.1038/nchem.1095 · Cited by 7,526
Photochemistry on Metal Nanoparticles
Watanabe, K., Menzel, D., Nilius, N., & Freund, H.-J. (2006) · Chemical Reviews · doi:10.1021/cr050167g · Cited by 486
The Power of Single‐Atom Catalysis
Liang, S., Hao, C., & Shi, Y. (2015) · ChemCatChem · doi:10.1002/cctc.201500363 · Cited by 365
The Multifaceted Reactivity of Single‐Atom Heterogeneous Catalysts
Mitchell, S., Vorobyeva, E., & Pérez‐Ramírez, J. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201806936 · Cited by 348
Serine Octamers: Cluster Formation, Reactions, and Implications for Biomolecule Homochirality
Nanita, S. C., & Cooks, R. G. (2006) · Angewandte Chemie International Edition · doi:10.1002/anie.200501328 · Cited by 184
Metadata
- Authors
- Böhme, D. K., & Schwarz, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2005-04-13
- Volume
- 44
- Issue
- 16
- Pages
- 2336-2354
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2073753357
- Cited by
- 856
- References
- 1
- FWCI
- 17.49
- Type
- journal article
- Language
- en
- Open access
- closed
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- Böhme, D. K., & Schwarz, H. (2005). Gas‐Phase Catalysis by Atomic and Cluster Metal Ions: The Ultimate Single‐Site Catalysts. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200461698
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