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Reversible Metal‐Free Carbon Dioxide Binding by Frustrated Lewis Pairs
Open accessAbstract
Hot and bothered? Frustrated Lewis pairs comprising phosphine and borane react to reversibly bind and release CO2, offering a rare example of metal-free CO2 sequestration. The mechanism of formation of these CO2 derivatives 1 and 2 (see scheme) by almost simultaneous PC and OB bond formation was characterized by quantum chemical calculations.
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Cited by
Frontiers, Opportunities, and Challenges in Biochemical and Chemical Catalysis of CO 2 Fixation
Appel, A. M., Bercaw, J. E., Bocarsly, A. B., Dobbek, H., DuBois, D. L., Dupuis, M., Ferry, J. G., Fujita, E., Hille, R., Kenis, P. J. A., et al. (2013) · Chemical Reviews · doi:10.1021/cr300463y · Cited by 2,193
Klankermayer, J., Wesselbaum, S., Beydoun, K., & Leitner, W. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201507458 · Cited by 856
Turning carbon dioxide into fuel
Jiang, Z., Xiao, T., Kuznetsov, V. L., & Edwards, P. P. (2010) · Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences · doi:10.1098/rsta.2010.0119 · Cited by 457
Photochemical Reduction of CO2 by Graphitic Carbon Nitride Polymers
Lin, J., Pan, Z., & Wang, X. (2014) · ACS Sustainable Chemistry & Engineering · doi:10.1021/sc4004295 · Cited by 409
Sorbents for CO2 capture from flue gas—aspects from materials and theoretical chemistry
Hedin, N., Chen, L., & Laaksonen, A. (2010) · Nanoscale · doi:10.1039/c0nr00042f · Cited by 243
Metadata
- Authors
- Mömming, C. M., Otten, E., Kehr, G., Fröhlich, R., Grimme, S., Stephan, D. W., & Erker, G.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2009-08-19
- Volume
- 48
- Issue
- 36
- Pages
- 6643-6646
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2171515789
- Cited by
- 770
- References
- 0
- FWCI
- 26.02
- Type
- journal article
- Language
- en
- Open access
- green
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- Mömming, C. M., Otten, E., Kehr, G., Fröhlich, R., Grimme, S., Stephan, D. W., & Erker, G. (2009). Reversible Metal‐Free Carbon Dioxide Binding by Frustrated Lewis Pairs. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200901636
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