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Oxygen Reactions in a Non‐Aqueous Li+ Electrolyte
Abstract
Taking the shortcut: Spectroscopic data (see picture) provide direct evidence that in non-aqueous Li+ electrolyte, O2 is reduced to O2−, which then forms LiO2 on the electrode surface which disproportionates to Li2O2. On charging, Li2O2 decomposes directly, in a one-step reaction to evolve O2 and does not pass through LiO2 as an intermediate.
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Citations
Cited by
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Self-citationElectrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Current density dependence of peroxide formation in the Li–O2 battery and its effect on charge
Adams, B. D., Radtke, C., Black, R., Trudeau, M. L., Zaghib, K., & Nazar, L. F. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40697k · Cited by 678
Catalytic Activity Trends of Oxygen Reduction Reaction for Nonaqueous Li-Air Batteries
Lu, Y.-C., Gasteiger, H. A., & Shao-Horn, Y. (2011) · Journal of the American Chemical Society · doi:10.1021/ja208608s · Cited by 567
Critical Challenges in Rechargeable Aprotic Li–O2 Batteries
Feng, N., He, P., & Zhou, H. (2016) · Advanced Energy Materials · doi:10.1002/aenm.201502303 · Cited by 423
Metadata
- Authors
- Peng, Z., Freunberger, S. A., Hardwick, L. J., Chen, Y., Giordani, V., Bardé, F., Novák, P., Graham, D., Tarascon, J., & Bruce, P. G.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2011-05-23
- Volume
- 50
- Issue
- 28
- Pages
- 6351-6355
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2136245070
- Cited by
- 595
- References
- 0
- FWCI
- 35.21
- Type
- journal article
- Language
- en
- Open access
- closed
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- Peng, Z., Freunberger, S. A., Hardwick, L. J., Chen, Y., Giordani, V., Bardé, F., Novák, P., Graham, D., Tarascon, J., & Bruce, P. G. (2011). Oxygen Reactions in a Non‐Aqueous Li+ Electrolyte. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201100879
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