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Chemical Activity of Thin Oxide Layers: Strong Interactions with the Support Yield a New Thin‐Film Phase of ZnO
Abstract
Influential support: Metal substrates affect the chemical properties of ZnO layers, which are important catalyst materials for the industrial production of methanol through the oxidation of CO. Interactions with the substrate lead to the formation of a new, planar ZnO thin-film phase, in which less highly oxidized Zn atoms bind CO more strongly than the Zn atoms in the normal wurtzite modification.
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Citations
Cited by
Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Lunkenbein, T., Schumann, J., Behrens, M., Schlögl, R., & Willinger, M. G. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201411581 · Cited by 608
Induced activation of the commercial Cu/ZnO/Al2O3 catalyst for the steam reforming of methanol
Li, D., Xu, F., Tang, X., Dai, S., Pu, T., Liu, X., Tian, P., Xuan, F., Xu, Z., Wachs, I. E., et al. (2022) · Nature Catalysis · doi:10.1038/s41929-021-00729-4 · Cited by 519
Wang, S., Ren, C., Tian, H., Yu, J., & Sun, M. (2018) · Physical Chemistry Chemical Physics · doi:10.1039/c8cp00808f · Cited by 423
Hydrogenation of CO2 to methanol and CO on Cu/ZnO/Al2O3: Is there a common intermediate or not?
Kunkes, E. L., Studt, F., Abild-Pedersen, F., Schlögl, R., & Behrens, M. (2015) · Journal of Catalysis · doi:10.1016/j.jcat.2014.12.016 · Cited by 349
Metadata
- Authors
- Schott, V., Oberhofer, H., Birkner, A., Xu, M., Wang, Y., Muhler, M., Reuter, K., & Wöll, C.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2013-09-17
- Volume
- 52
- Issue
- 45
- Pages
- 11925-11929
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4249261575
- Cited by
- 198
- References
- 0
- FWCI
- 5.33
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Schott, V., Oberhofer, H., Birkner, A., Xu, M., Wang, Y., Muhler, M., Reuter, K., & Wöll, C. (2013). Chemical Activity of Thin Oxide Layers: Strong Interactions with the Support Yield a New Thin‐Film Phase of ZnO. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201302315
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