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Well‐Defined Metal–Organic Framework Hollow Nanocages
Abstract
Metal–organic frameworks (MOFs) have demonstrated great potentials in a variety of important applications. To enhance the inherent properties and endow materials with multifunctionality, the rational design and synthesis of MOFs with nanoscale porosity and hollow feature is highly desired and remains a great challenge. In this work, the formation of a series of well‐defined MOF (MOF‐5, Fe II‐MOF‐5, Fe III‐MOF‐5) hollow nanocages by a facile solvothermal method, without any additional supporting template is reported. A surface‐energy‐driven mechanism may be responsible for the formation of hollow nanocages. The addition of pre‐synthesized poly(vinylpyrrolidone)‐ (PVP) capped noble‐metal nanoparticles into the synthetic system of MOF hollow nanocages yields the yolk–shell noble metal@MOF nanostructures. The present strategy to fabricate hollow and yolk–shell nanostructures is expected to open up exciting opportunities for developing a novel class of inorganic–organic hybrid functional nanomaterials.
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Cited by
Synthesis, Properties, and Applications of Hollow Micro-/Nanostructures
Wang, X., Feng, J., Bai, Y., Zhang, Q., & Yin, Y. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00731 · Cited by 1,456
Self-citationJiang, R., Li, L., Sheng, T., Hu, G., Chen, Y., & Wang, L. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b07294 · Cited by 797
Self-citationHan, L., Yu, X., & Lou, X. W. (. (2016) · Advanced Materials · doi:10.1002/adma.201506315 · Cited by 633
Chen, Y.-Z., Zhou, Y.-X., Wang, H., Lu, J., Uchida, T., Xu, Q., Yu, S.-H., & Jiang, H.-L. (2015) · ACS Catalysis · doi:10.1021/cs501953d · Cited by 423
Self-citationMulti‐shelled Hollow Metal–Organic Frameworks
Liu, W., Huang, J., Yang, Q., Wang, S., Sun, X., Zhang, W., Liu, J., & Huo, F. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201701604 · Cited by 367
Metadata
- Authors
- Zhang, Z., Chen, Y., Xu, X., Zhang, J., Xiang, G., He, W., & Wang, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2013-11-28
- Volume
- 53
- Issue
- 2
- Pages
- 429-433
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2156389261
- Cited by
- 350
- References
- 0
- FWCI
- 14.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, Z., Chen, Y., Xu, X., Zhang, J., Xiang, G., He, W., & Wang, X. (2014). Well‐Defined Metal–Organic Framework Hollow Nanocages. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201308589
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