The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
High‐Yield Electrochemical Production of Formaldehyde from CO2 and Seawater
Abstract
The catalytic, electrocatalytic, or photocatalytic conversion of CO 2 into useful chemicals in high yield for industrial applications has so far proven difficult. Herein, we present our work on the electrochemical reduction of CO 2 in seawater using a boron‐doped diamond (BDD) electrode under ambient conditions to produce formaldehyde. This method overcomes the usual limitation of the low yield of higher‐order products, and also reduces the generation of H 2. In comparison with other electrode materials, BDD electrodes have a wide potential window and high electrochemical stability, and, moreover, exhibit very high Faradaic efficiency (74 %) for the production of formaldehyde, using either methanol, aqueous NaCl, or seawater as the electrolyte. The high Faradaic efficiency is attributed to the sp 3‐bonded carbon of the BDD. Our results have wide ranging implications for the efficient and cost‐effective conversion of CO 2.
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Cites
Ionic Liquid–Mediated Selective Conversion of CO 2 to CO at Low Overpotentials
Rosen, B. A., Salehi-Khojin, A., Thorson, M. R., Zhu, W., Whipple, D. T., Kenis, P. J. A., & Masel, R. I. (2011) · Science · doi:10.1126/science.1209786 · Cited by 1,558
Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
Zhang, L., Zhao, Z., & Gong, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201612214 · Cited by 1,048
CO2 Reduction: From the Electrochemical to Photochemical Approach
Wu, J., Huang, Y., Ye, W., & Li, Y. (2017) · Advanced Science · doi:10.1002/advs.201700194 · Cited by 937
Oxygen Vacancies in ZnO Nanosheets Enhance CO2 Electrochemical Reduction to CO
Geng, Z., Kong, X., Chen, W., Su, H., Liu, Y., Cai, F., Wang, G., & Zeng, J. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201711255 · Cited by 771
Metal‐Free Carbon Materials for CO2 Electrochemical Reduction
Duan, X., Xu, J., Wei, Z., Ma, J., Guo, S., Wang, S., Liu, H., & Dou, S. (2017) · Advanced Materials · doi:10.1002/adma.201701784 · Cited by 754
Metadata
- Authors
- Nakata, K., Ozaki, T., Terashima, C., Fujishima, A., & Einaga, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2013-11-26
- Volume
- 53
- Issue
- 3
- Pages
- 871-874
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2126197024
- Cited by
- 410
- References
- 1
- FWCI
- 6.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- Nakata, K., Ozaki, T., Terashima, C., Fujishima, A., & Einaga, Y. (2014). High‐Yield Electrochemical Production of Formaldehyde from CO2 and Seawater. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201308657
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