The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Metal‐Doped Nitrogenated Carbon as an Efficient Catalyst for Direct CO2 Electroreduction to CO and Hydrocarbons
Abstract
This study explores the kinetics, mechanism, and active sites of the CO 2 electroreduction reaction (CO2RR) to syngas and hydrocarbons on a class of functionalized solid carbon‐based catalysts. Commercial carbon blacks were functionalized with nitrogen and Fe and/or Mn ions using pyrolysis and acid leaching. The resulting solid powder catalysts were found to be active and highly CO selective electrocatalysts in the electroreduction of CO 2 to CO/H 2 mixtures outperforming a low‐area polycrystalline gold benchmark. Unspecific with respect to the nature of the metal, CO production is believed to occur on nitrogen functionalities in competition with hydrogen evolution. Evidence is provided that sufficiently strong interaction between CO and the metal enables the protonation of CO and the formation of hydrocarbons. Our results highlight a promising new class of low‐cost, abundant electrocatalysts for synthetic fuel production from CO 2.
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Cites
High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
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How copper catalyzes the electroreduction of carbon dioxide into hydrocarbon fuels
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New insights into the electrochemical reduction of carbon dioxide on metallic copper surfaces
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Electrocatalytic Conversion of Carbon Dioxide to Methane and Methanol on Transition Metal Surfaces
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Self-citationCompetition between CO 2 Reduction and H 2 Evolution on Transition-Metal Electrocatalysts
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Nitrogen-Based Catalysts for the Electrochemical Reduction of CO 2 to CO
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
Domino electroreduction of CO2 to methanol on a molecular catalyst
Wu, Y., Jiang, Z., Lu, X., Liang, Y., & Wang, H. (2019) · Nature · doi:10.1038/s41586-019-1760-8 · Cited by 1,194
Large-Scale and Highly Selective CO2 Electrocatalytic Reduction on Nickel Single-Atom Catalyst
Zheng, T., Jiang, K., Ta, N., Hu, Y., Zeng, J., Liu, J., & Wang, H. (2019) · Joule · doi:10.1016/j.joule.2018.10.015 · Cited by 887
Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Jiang, K., Siahrostami, S., Akey, A. J., Li, Y., Lu, Z., Lattimer, J., Hu, Y., Stokes, C., Gangishetty, M., Chen, G., et al. (2017) · Chem · doi:10.1016/j.chempr.2017.09.014 · Cited by 406
Metadata
- Authors
- Varela, A. S., Ranjbar Sahraie, N., Steinberg, J., Ju, W., Oh, H., & Strasser, P.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-07-29
- Volume
- 54
- Issue
- 37
- Pages
- 10758-10762
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2155563668
- Cited by
- 618
- References
- 10
- FWCI
- 11.63
- Type
- journal article
- Language
- en
- Open access
- closed
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- Varela, A. S., Ranjbar Sahraie, N., Steinberg, J., Ju, W., Oh, H., & Strasser, P. (2015). Metal‐Doped Nitrogenated Carbon as an Efficient Catalyst for Direct CO2 Electroreduction to CO and Hydrocarbons. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201502099
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