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Methylamine‐Gas‐Induced Defect‐Healing Behavior of CH3NH3PbI3 Thin Films for Perovskite Solar Cells
Abstract
We report herein the discovery of methylamine (CH 3 NH 2) induced defect‐healing (MIDH) of CH 3 NH 3 PbI 3 perovskite thin films based on their ultrafast (seconds), reversible chemical reaction with CH 3 NH 2 gas at room temperature. The key to this healing behavior is the formation and spreading of an intermediate CH 3 NH 3 PbI 3⋅x CH 3 NH 2 liquid phase during this unusual perovskite–gas interaction. We demonstrate the versatility and scalability of the MIDH process, and show dramatic enhancement in the performance of perovskite solar cells (PSCs) with MIDH. This study represents a new direction in the formation of defect‐free films of hybrid perovskites.
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Kim, H.-S., Lee, C.-R., Im, J.-H., Lee, K.-B., Moehl, T., Marchioro, A., Moon, S.-J., Humphry-Baker, R., Yum, J.-H., Moser, J. E., et al. (2012) · Scientific Reports · doi:10.1038/srep00591 · Cited by 8,092
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
Cited by
Brenner, T. M., Egger, D. A., Kronik, L., Hodes, G., & Cahen, D. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.7 · Cited by 1,557
Scalable fabrication and coating methods for perovskite solar cells and solar modules
Park, N.-G., & Zhu, K. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0176-2 · Cited by 908
Ke, W., Xiao, C., Wang, C., Saparov, B., Duan, H., Zhao, D., Xiao, Z., Schulz, P., Harvey, S. P., Liao, W., et al. (2016) · Advanced Materials · doi:10.1002/adma.201600594 · Cited by 579
Li, G., She, C., Zhang, Y., Li, H., Liu, S., Yue, F., Jing, C., Cheng, Y., & Chu, J. (2021) · Sensors and Actuators B: Chemical · doi:10.1016/j.snb.2020.128918 · Cited by 60
Brintakis, K., Gagaoudakis, E., Kostopoulou, A., Faka, V., Argyrou, A., Binas, V., Kiriakidis, G., & Stratakis, E. (2019) · Nanoscale Advances · doi:10.1039/c9na00219g · Cited by 58
Metadata
- Authors
- Zhou, Z., Wang, Z., Zhou, Y., Pang, S., Wang, D., Xu, H., Liu, Z., Padture, N. P., & Cui, G.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-06-26
- Volume
- 54
- Issue
- 33
- Pages
- 9705-9709
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2166662984
- Cited by
- 440
- References
- 2
- FWCI
- 29.03
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Zhou, Z., Wang, Z., Zhou, Y., Pang, S., Wang, D., Xu, H., Liu, Z., Padture, N. P., & Cui, G. (2015). Methylamine‐Gas‐Induced Defect‐Healing Behavior of CH3NH3PbI3 Thin Films for Perovskite Solar Cells. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201504379
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