The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Ultrathin Co3O4 Layers Realizing Optimized CO2 Electroreduction to Formate
Abstract
Electroreduction of CO 2 into hydrocarbons could contribute to alleviating energy crisis and global warming. However, conventional electrocatalysts usually suffer from low energetic efficiency and poor durability. Herein, atomic layers for transition‐metal oxides are proposed to address these problems through offering an ultralarge fraction of active sites, high electronic conductivity, and superior structural stability. As a prototype, 1.72 and 3.51 nm thick Co 3 O 4 layers were synthesized through a fast‐heating strategy. The atomic thickness endowed Co 3 O 4 with abundant active sites, ensuring a large CO 2 adsorption amount. The increased and more dispersed charge density near Fermi level allowed for enhanced electronic conductivity. The 1.72 nm thick Co 3 O 4 layers showed over 1.5 and 20 times higher electrocatalytic activity than 3.51 nm thick Co 3 O 4 layers and bulk counterpart, respectively. Also, 1.72 nm thick Co 3 O 4 layers showed formate Faradaic efficiency of over 60 % in 20 h.
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Cites
Li, C. W., & Kanan, M. W. (2012) · Journal of the American Chemical Society · doi:10.1021/ja3010978 · Cited by 2,000
Electroreduction of carbon monoxide to liquid fuel on oxide-derived nanocrystalline copper
Li, C. W., Ciston, J., & Kanan, M. W. (2014) · Nature · doi:10.1038/nature13249 · Cited by 1,728
Ionic Liquid–Mediated Selective Conversion of CO 2 to CO at Low Overpotentials
Rosen, B. A., Salehi-Khojin, A., Thorson, M. R., Zhu, W., Whipple, D. T., Kenis, P. J. A., & Masel, R. I. (2011) · Science · doi:10.1126/science.1209786 · Cited by 1,558
Active and Selective Conversion of CO 2 to CO on Ultrathin Au Nanowires
Zhu, W., Zhang, Y.-J., Zhang, H., Lv, H., Li, Q., Michalsky, R., Peterson, A. A., & Sun, S. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5095099 · Cited by 860
Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
Fundamentals and challenges of electrochemical CO2 reduction using two-dimensional materials
Sun, Z., Ma, T., Tao, H., Fan, Q., & Han, B. (2017) · Chem · doi:10.1016/j.chempr.2017.09.009 · Cited by 1,224
Self-citationElectrocatalytic reduction of nitrate – a step towards a sustainable nitrogen cycle
Xu, H., Ma, Y., Chen, J., Zhang, W.-X., & Yang, J. (2022) · Chemical Society Reviews · doi:10.1039/d1cs00857a · Cited by 1,160
Self-citationZhang, L., Zhao, Z., & Gong, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201612214 · Cited by 1,048
Jiao, X., Chen, Z., Li, X., Sun, Y., Gao, S., Yan, W., Wang, C., Zhang, Q., Lin, Y., Luo, Y., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b02290 · Cited by 1,049
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Metadata
- Authors
- Gao, S., Jiao, X., Sun, Z., Zhang, W., Sun, Y., Wang, C., Hu, Q., Zu, X., Yang, F., Yang, S., Liang, L., Wu, J., & Xie, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-11-24
- Volume
- 55
- Issue
- 2
- Pages
- 698-702
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2179368292
- Cited by
- 481
- References
- 4
- FWCI
- 12.61
- Type
- journal article
- Language
- en
- Open access
- closed
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- Gao, S., Jiao, X., Sun, Z., Zhang, W., Sun, Y., Wang, C., Hu, Q., Zu, X., Yang, F., Yang, S., Liang, L., Wu, J., & Xie, Y. (2016). Ultrathin Co3O4 Layers Realizing Optimized CO2 Electroreduction to Formate. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201509800
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