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Stabilizing a Platinum1 Single‐Atom Catalyst on Supported Phosphomolybdic Acid without Compromising Hydrogenation Activity
Open accessAbstract
In coordination chemistry, catalytically active metal complexes in a zero‐ or low‐valent state often adopt four‐coordinate square‐planar or tetrahedral geometry. By applying this principle, we have developed a stable Pt 1 single‐atom catalyst with a high Pt loading (close to 1 wt %) on phosphomolybdic acid(PMA)‐modified active carbon. This was achieved by anchoring Pt on the four‐fold hollow sites on PMA. Each Pt atom is stabilized by four oxygen atoms in a distorted square‐planar geometry, with Pt slightly protruding from the oxygen planar surface. Pt is positively charged, absorbs hydrogen easily, and exhibits excellent performance in the hydrogenation of nitrobenzene and cyclohexanone. It is likely that the system described here can be extended to a number of stable SACs with superior catalytic activities.
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A fast and robust algorithm for Bader decomposition of charge density
Henkelman, G., Arnaldsson, A., & Jónsson, H. (2006) · Computational Materials Science · doi:10.1016/j.commatsci.2005.04.010 · Cited by 10,723
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
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Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Single Pt Atoms Confined into a Metal–Organic Framework for Efficient Photocatalysis
Fang, X., Shang, Q., Wang, Y., Jiao, L., Yao, T., Li, Y., Zhang, Q., Luo, Y., & Jiang, H. (2018) · Advanced Materials · doi:10.1002/adma.201705112 · Cited by 837
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The Multifaceted Reactivity of Single‐Atom Heterogeneous Catalysts
Mitchell, S., Vorobyeva, E., & Pérez‐Ramírez, J. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201806936 · Cited by 348
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Metadata
- Authors
- Zhang, B., Asakura, H., Zhang, J., Zhang, J., De, S., & Yan, N.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-05-30
- Volume
- 55
- Issue
- 29
- Pages
- 8319-8323
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2415897117
- Cited by
- 422
- References
- 3
- FWCI
- 24.65
- Type
- journal article
- Language
- en
- Open access
- green
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- Zhang, B., Asakura, H., Zhang, J., Zhang, J., De, S., & Yan, N. (2016). Stabilizing a Platinum1 Single‐Atom Catalyst on Supported Phosphomolybdic Acid without Compromising Hydrogenation Activity. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201602801
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