The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Organic Polymer Dots as Photocatalysts for Visible Light‐Driven Hydrogen Generation
Open accessAbstract
For the first time, organic semiconducting polymer dots (Pdots) based on poly[(9,9′‐dioctylfluorenyl‐2,7‐diyl)‐co‐(1,4‐benzo‐{2,1′,3} thiadiazole)] (PFBT) and polystyrene grafting with carboxyl‐group‐functionalized ethylene oxide (PS‐PEG‐COOH) are introduced as a photocatalyst towards visible‐light‐driven hydrogen generation in a completely organic solvent‐free system. With these organic Pdots as the photocatalyst, an impressive initial rate constant of 8.3 mmol h−1 g−1 was obtained for visible‐light‐driven hydrogen production, which is 5‐orders of magnitude higher than that of pristine PFBT polymer under the same catalytic conditions. Detailed kinetics studies suggest that the productive electron transfer quench of the excited state of Pdots by an electron donor is about 40 %. More importantly, we also found that the Pdots can tolerate oxygen during catalysis, which is crucial for further application of this material for light‐driven water splitting.
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Opportunities and challenges for a sustainable energy future
Chu, S., & Majumdar, A. (2012) · Nature · doi:10.1038/nature11475 · Cited by 12,550
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Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Cited by
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Sharma, R. K., Yadav, P., Yadav, M., Gupta, R., Rana, P., Srivastava, A., Zbořil, R., Varma, R. S., Antonietti, M., & Gawande, M. B. (2020) · Materials Horizons · doi:10.1039/c9mh00856j · Cited by 455
Bao, X., Yuan, Y., Chen, J., Zhang, B., Li, D., Zhou, D., Jing, P., Xu, G., Wang, Y., Holá, K., et al. (2018) · Light: Science & Applications · doi:10.1038/s41377-018-0090-1 · Cited by 445
Bai, Y., Wilbraham, L., Slater, B. J., Zwijnenburg, M. A., Sprick, R. S., & Cooper, A. I. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03591 · Cited by 409
Metadata
- Authors
- Wang, L., Fernández‐Terán, R., Zhang, L., Fernandes, D. L. A., Tian, L., Chen, H., & Tian, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-09-08
- Volume
- 55
- Issue
- 40
- Pages
- 12306-12310
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2515163590
- Cited by
- 255
- References
- 3
- FWCI
- 6.26
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Wang, L., Fernández‐Terán, R., Zhang, L., Fernandes, D. L. A., Tian, L., Chen, H., & Tian, H. (2016). Organic Polymer Dots as Photocatalysts for Visible Light‐Driven Hydrogen Generation. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201607018
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