The DOI matches its Crossref record; 62 of the 62 references it cites were found in a registry or an index.
Crystallinity‐Modulated Electrocatalytic Activity of a Nickel(II) Borate Thin Layer on Ni3B for Efficient Water Oxidation
Abstract
The exploration of new efficient OER electrocatalysts based on nonprecious metals and the understanding of the relationship between activity and structure of electrocatalysts are important to advance electrochemical water oxidation. Herein, we developed an efficient OER electrocatalyst with nickel boride (Ni 3 B) nanoparticles as cores and nickel(II) borate (Ni‐B i) as shells (Ni‐B i@NB) via a very simple and facile aqueous reaction. This electrocatalyst exhibited a small overpotential of 302 mV at 10 mA cm−2 and Tafel slope of 52 mV dec−1. More interestingly, it was found that the OER activity of Ni‐B i@NB was closely dependent on the crystallinity of the Ni‐B i shells. The partially crystalline Ni‐B i catalyst exhibited much higher activity than the amorphous or crystalline analogues; this higher activity originated from the enhanced intrinsic activity of the catalytic sites. These findings open up opportunities to explore nickel(II) borates as a new class of efficient nonprecious metal OER electrocatalysts, and to improve the electrocatalyst performance by modulating their crystallinity.
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Cites
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Cited by
Liu, D., Ai, H., Li, J., Fang, M., Chen, M., Liu, D., Du, X., Zhou, P., Li, F., Lo, K. H., et al. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202002464 · Cited by 303
Self-citationWang, X., Ma, W., Ding, C., Xu, Z., Wang, H., Zong, X., & Li, C. (2018) · ACS Catalysis · doi:10.1021/acscatal.8b01839 · Cited by 168
Development Strategies in Transition Metal Borides for Electrochemical Water Splitting
Yao, Y., Zhang, Z., & Jiao, L. (2022) · ENERGY & ENVIRONMENTAL MATERIALS · doi:10.1002/eem2.12198 · Cited by 138
Electrocatalytic Upgrading of Lignin‐Derived Bio‐Oil Based on Surface‐Engineered PtNiB Nanostructure
Zhou, Y., Gao, Y., Zhong, X., Jiang, W., Liang, Y., Niu, P., Li, M., Zhuang, G., Li, X., & Wang, J. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201807651 · Cited by 136
Self-citationZhao, W., Xu, T., Li, T., Wang, Y., Liu, H., Feng, J., Ding, S., Li, Z., & Wu, M. (2018) · Small · doi:10.1002/smll.201802829 · Cited by 59
Metadata
- Authors
- Jiang, W., Niu, S., Tang, T., Zhang, Q., Liu, X., Zhang, Y., Chen, Y., Li, J., Gu, L., Wan, L., & Hu, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-05-04
- Volume
- 56
- Issue
- 23
- Pages
- 6572-6577
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2610884856
- Cited by
- 346
- References
- 62
- FWCI
- 11.17
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jiang, W., Niu, S., Tang, T., Zhang, Q., Liu, X., Zhang, Y., Chen, Y., Li, J., Gu, L., Wan, L., & Hu, J. (2017). Crystallinity‐Modulated Electrocatalytic Activity of a Nickel(II) Borate Thin Layer on Ni3B for Efficient Water Oxidation. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201703183
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