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An Intrinsically Stretchable and Compressible Supercapacitor Containing a Polyacrylamide Hydrogel Electrolyte
Abstract
Stretchability and compressibility of supercapacitors is an essential element of modern electronics, such as flexible, wearable devices. Widely used polyvinyl alcohol‐based electrolytes are neither very stretchable nor compressible, which fundamentally limits the realization of supercapacitors with high stretchability and compressibility. A new electrolyte that is intrinsically super‐stretchable and compressible is presented. Vinyl hybrid silica nanoparticle cross‐linkers were introduced into polyacrylamide hydrogel backbones to promote dynamic cross‐linking of the polymer networks. These cross‐linkers serve as stress buffers to dissipate energy when strain is applied, providing a solution to the intrinsically low stretchability and compressibility shortcomings of conventional supercapacitors. The newly developed supercapacitor and electrolyte can be stretched up to an unprecedented 1000 % strain with enhanced performance, and compressed to 50 % strain with good retention of the initial performance.
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Kim, D.-H., Lu, N., Ma, R., Kim, Y.-S., Kim, R.-H., Wang, S., Wu, J., Won, S. M., Tao, H., Islam, A., et al. (2011) · Science · doi:10.1126/science.1206157 · Cited by 4,836
Self-citationHighly stretchable electroluminescent skin for optical signaling and tactile sensing
Larson, C., Peele, B., Li, S., Robinson, S., Totaro, M., Beccai, L., Mazzolai, B., & Shepherd, R. (2016) · Science · doi:10.1126/science.aac5082 · Cited by 1,393
Cited by
Gel Polymer Electrolytes for Electrochemical Energy Storage
Cheng, X., Pan, J., Zhao, Y., Liao, M., & Peng, H. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702184 · Cited by 1,020
Li, H., Liu, Z., Liang, G., Huang, Y., Huang, Y., Zhu, M., Pei, Z., Xue, Q., Tang, Z., Wang, Y., et al. (2018) · ACS Nano · doi:10.1021/acsnano.7b09003 · Cited by 587
Self-citationDing, Q., Xu, X., Yue, Y., Mei, C., Huang, C., Jiang, S., Wu, Q., & Han, J. (2018) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.8b09656 · Cited by 518
Beyond Charge Balance: Counter‐Cations in Polyoxometalate Chemistry
Misra, A., Kozma, K., Streb, C., & Nyman, M. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201905600 · Cited by 482
From design to applications of stimuli-responsive hydrogel strain sensors
Zhang, D., Ren, B., Zhang, Y., Xu, L., Huang, Q., He, Y., Li, X., Wu, J., Yang, J., Chen, Q., et al. (2020) · Journal of Materials Chemistry B · doi:10.1039/c9tb02692d · Cited by 199
Metadata
- Authors
- Huang, Y., Zhong, M., Shi, F., Liu, X., Tang, Z., Wang, Y., Huang, Y., Hou, H., Xie, X., & Zhi, C.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-06-29
- Volume
- 56
- Issue
- 31
- Pages
- 9141-9145
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2631900311
- Cited by
- 563
- References
- 2
- FWCI
- 21.10
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, Y., Zhong, M., Shi, F., Liu, X., Tang, Z., Wang, Y., Huang, Y., Hou, H., Xie, X., & Zhi, C. (2017). An Intrinsically Stretchable and Compressible Supercapacitor Containing a Polyacrylamide Hydrogel Electrolyte. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201705212
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