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Fe‐Doped Ni3C Nanodots in N‐Doped Carbon Nanosheets for Efficient Hydrogen‐Evolution and Oxygen‐Evolution Electrocatalysis
Abstract
Uniform Ni 3 C nanodots dispersed in ultrathin N‐doped carbon nanosheets were successfully prepared by carburization of the two dimensional (2D) nickel cyanide coordination polymer precursors. The Ni 3 C based nanosheets have lateral length of about 200 nm and thickness of 10 nm. When doped with Fe, the Ni 3 C based nanosheets exhibited outstanding electrocatalytic properties for both the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). For example, 2 at % Fe (atomic percent) doped Ni 3 C nanosheets depict a low overpotential (292 mV) and a small Tafel slope (41.3 mV dec−1) for HER in KOH solution. An outstanding OER catalytic property is also achieved with a low overpotential of 275 mV and a small Tafel slope of 62 mV dec−1 in KOH solution. Such nanodot‐incorporated 2D hybrid structures can serve as an efficient bifunctional electrocatalyst for overall water splitting.
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Cited by
Recent Advances in Electrocatalytic Hydrogen Evolution Using Nanoparticles
Zhu, J., Hu, L., Zhao, P., Lee, L. Y. S., & Wong, K.-Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00248 · Cited by 3,133
Anantharaj, S., Kundu, S., & Noda, S. (2021) · Nano Energy · doi:10.1016/j.nanoen.2020.105514 · Cited by 932
Ouyang, T., Ye, Y., Wu, C., Xiao, K., & Liu, Z. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201814262 · Cited by 804
Gao, Q., Zhang, W., Shi, Z., Yang, L., & Tang, Y. (2019) · Advanced Materials · doi:10.1002/adma.201802880 · Cited by 734
Zhu, K., Zhu, X., & Yang, W. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201802923 · Cited by 721
Metadata
- Authors
- Fan, H., Yu, H., Zhang, Y., Zheng, Y., Luo, Y., Dai, Z., Li, B., Zong, Y., & Yan, Q.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-09-05
- Volume
- 56
- Issue
- 41
- Pages
- 12566-12570
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2746949191
- Cited by
- 387
- References
- 0
- FWCI
- 12.74
- Type
- journal article
- Language
- en
- Open access
- closed
- Funders
- Singapore MOE Tier 1 (2016-T1-002-065, RG113/15)
- Singapore EMA (EIRP 12/NRF2015EWT-EIRP002-008)
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- Fan, H., Yu, H., Zhang, Y., Zheng, Y., Luo, Y., Dai, Z., Li, B., Zong, Y., & Yan, Q. (2017). Fe‐Doped Ni3C Nanodots in N‐Doped Carbon Nanosheets for Efficient Hydrogen‐Evolution and Oxygen‐Evolution Electrocatalysis. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201706610
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