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Biocatalytic Oxidation Reactions: A Chemist's Perspective
Open accessAbstract
Oxidation chemistry using enzymes is approaching maturity and practical applicability in organic synthesis. Oxidoreductases (enzymes catalysing redox reactions) enable chemists to perform highly selective and efficient transformations ranging from simple alcohol oxidations to stereoselective halogenations of non‐activated C−H bonds. For many of these reactions, no “classical” chemical counterpart is known. Hence oxidoreductases open up shorter synthesis routes based on a more direct access to the target products. The generally very mild reaction conditions may also reduce the environmental impact of biocatalytic reactions compared to classical counterparts. In this Review, we critically summarise the most important recent developments in the field of biocatalytic oxidation chemistry and identify the most pressing bottlenecks as well as promising solutions.
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Cited by
Cytochrome P450 Monooxygenases in Biotechnology and Synthetic Biology
Urlacher, V. B., & Girhard, M. (2019) · Trends in Biotechnology · doi:10.1016/j.tibtech.2019.01.001 · Cited by 355
Ivshina, I., Bazhutin, G., & Tyumina, E. (2022) · Frontiers in Microbiology · doi:10.3389/fmicb.2022.967127 · Cited by 62
The Evolution and Evolvability of Photosystem II
Oliver, T., Kim, T. D., Trinugroho, J. P., Cordón-Preciado, V., Wijayatilake, N., Bhatia, A., Rutherford, A. W., & Cardona, T. (2023) · Annual Review of Plant Biology · doi:10.1146/annurev-arplant-070522-062509 · Cited by 52
Metadata
- Authors
- Dong, J., Fernández‐Fueyo, E., Hollmann, F., Paul, C. E., Pesic, M., Schmidt, S., Wang, Y., Younes, S., & Zhang, W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-07-03
- Volume
- 57
- Issue
- 30
- Pages
- 9238-9261
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2810361637
- Cited by
- 479
- References
- 0
- FWCI
- 17.11
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- The paper
- Dong, J., Fernández‐Fueyo, E., Hollmann, F., Paul, C. E., Pesic, M., Schmidt, S., Wang, Y., Younes, S., & Zhang, W. (2018). Biocatalytic Oxidation Reactions: A Chemist's Perspective. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201800343
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