The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Tuning Cu/Cu2O Interfaces for the Reduction of Carbon Dioxide to Methanol in Aqueous Solutions
Abstract
Artificial photosynthesis can be used to store solar energy and reduce CO 2 into fuels to potentially alleviate global warming and the energy crisis. Compared to the generation of gaseous products, it remains a great challenge to tune the product distribution of artificial photosynthesis to liquid fuels, such as CH 3 OH, which are suitable for storage and transport. Herein, we describe the introduction of metallic Cu nanoparticles (NPs) on Cu 2 O films to change the product distribution from gaseous products on bare Cu 2 O to predominantly CH 3 OH by CO 2 reduction in aqueous solutions. The specifically designed Cu/Cu 2 O interfaces balance the binding strengths of H* and CO* intermediates, which play critical roles in CH 3 OH production. With a TiO 2 model photoanode to construct a photoelectrochemical cell, a Cu/Cu 2 O dark cathode exhibited a Faradaic efficiency of up to 53.6 % for CH 3 OH production. This work demonstrates the feasibility and mechanism of interface engineering to enhance the CH 3 OH production from CO 2 reduction in aqueous electrolytes.
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Cites
How copper catalyzes the electroreduction of carbon dioxide into hydrocarbon fuels
Peterson, A. A., Abild-Pedersen, F., Studt, F., Rossmeisl, J., & Nørskov, J. K. (2010) · Energy & Environmental Science · doi:10.1039/c0ee00071j · Cited by 3,784
Ulissi, Z. W., Tang, M. T., Xiao, J., Liu, X., Torelli, D. A., Karamad, M., Cummins, K., Hahn, C., Lewis, N. S., Jaramillo, T. F., et al. (2017) · ACS Catalysis · doi:10.1021/acscatal.7b01648 · Cited by 387
Lee, S., Kim, D., & Lee, J. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201505730 · Cited by 320
Cited by
Ma, W., Xie, S., Liu, T., Fan, Q., Ye, J., Sun, F., Jiang, Z., Zhang, Q., Cheng, J., & Wang, Y. (2020) · Nature Catalysis · doi:10.1038/s41929-020-0450-0 · Cited by 1,468
Gong, Z., Zhong, W., He, Z., Liu, Q., Chen, H., Zhou, D., Zhang, N., Kang, X., & Chen, Y. (2022) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2021.121021 · Cited by 283
Self-citationHu, Q., Han, Z., Wang, X., Li, G., Wang, Z., Huang, X., Yang, H., Ren, X., Zhang, Q., Liu, J., et al. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202009277 · Cited by 241
Interface-Engineered Cu/Cu2In Metallic Aerogels for Efficient Electrochemical CO2 Reduction
Chen, C., Huang, H., Chen, Y., Zhang, Z., Fu, H., Li, H., Huang, W.-H., Lai, F., Zhang, N., & Liu, T. (2024) · ACS Materials Letters · doi:10.1021/acsmaterialslett.3c01473 · Cited by 14
Metadata
- Authors
- Chang, X., Wang, T., Zhao, Z., Yang, P., Greeley, J., Mu, R., Zhang, G., Gong, Z., Luo, Z., Chen, J., Cui, Y., Ozin, G. A., & Gong, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-10-31
- Volume
- 57
- Issue
- 47
- Pages
- 15415-15419
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2896294412
- Cited by
- 235
- References
- 3
- FWCI
- 6.67
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chang, X., Wang, T., Zhao, Z., Yang, P., Greeley, J., Mu, R., Zhang, G., Gong, Z., Luo, Z., Chen, J., Cui, Y., Ozin, G. A., & Gong, J. (2018). Tuning Cu/Cu2O Interfaces for the Reduction of Carbon Dioxide to Methanol in Aqueous Solutions. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201805256
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