The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
In Situ Thermal Atomization To Convert Supported Nickel Nanoparticles into Surface‐Bound Nickel Single‐Atom Catalysts
Abstract
The arrangement of the active sites on the surface of a catalysts can reduce the problem of mass transfer and enhance the atom economy. Herein, supported Ni metal nanoparticles can be transformed to thermal stable Ni single atoms, mostly located on the surface of the support. Assisted by N‐doped carbon with abundant defects, this synthetic process not only transform the nanoparticles to single atoms, but also creates numerous pores to facilitate the contact of dissolved CO 2 and single Ni sites. The proposed mechanism is that the Ni nanoparticles could break surface C−C bonds drill into the carbon matrix, leaving pores on the surface. When Ni nanoparticles are exposed to N‐doped carbon, the strong coordination splits Ni atoms from Ni NPs. The Ni atoms are stabilized within the surface of carbon substrate. The continuous loss of atomic Ni species from the NPs would finally result in atomization of Ni NPs. CO 2 electroreduction testing shows that the surface enriched with Ni single atoms delivers better performance than supported Ni NPs and other similar catalysts.
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Cites
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
Qiao, J., Liu, Y., Hong, F., & Zhang, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60323g · Cited by 2,990
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
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Self-citationPartially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Self-citationElectroreduction of carbon monoxide to liquid fuel on oxide-derived nanocrystalline copper
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications
Gao, C., Low, J., Long, R., Kong, T., Zhu, J., & Xiong, Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00840 · Cited by 1,050
Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Self-citationLu, X. F., Fang, Y., Luan, D., & Lou, X. W. D. (2021) · Nano Letters · doi:10.1021/acs.nanolett.0c04898 · Cited by 555
Recent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
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Metadata
- Authors
- Yang, J., Qiu, Z., Zhao, C., Wei, W., Chen, W., Li, Z., Qu, Y., Dong, J., Luo, J., Li, Z., & Wu, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-10
- Volume
- 57
- Issue
- 43
- Pages
- 14095-14100
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2891613004
- Cited by
- 422
- References
- 6
- FWCI
- 10.63
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, J., Qiu, Z., Zhao, C., Wei, W., Chen, W., Li, Z., Qu, Y., Dong, J., Luo, J., Li, Z., & Wu, Y. (2018). In Situ Thermal Atomization To Convert Supported Nickel Nanoparticles into Surface‐Bound Nickel Single‐Atom Catalysts. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201808049
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