The DOI matches its Crossref record; 34 of the 34 references it cites were found in a registry or an index.
Efficient Electrochemical Reduction of CO2 to HCOOH over Sub‐2 nm SnO2 Quantum Wires with Exposed Grain Boundaries
Open accessAbstract
Electrochemical reduction of CO 2 could mitigate environmental problems originating from CO 2 emission. Although grain boundaries (GBs) have been tailored to tune binding energies of reaction intermediates and consequently accelerate the CO 2 reduction reaction (CO 2 RR), it is challenging to exclusively clarify the correlation between GBs and enhanced reactivity in nanostructured materials with small dimension (<10 nm). Now, sub‐2 nm SnO 2 quantum wires (QWs) composed of individual quantum dots (QDs) and numerous GBs on the surface were synthesized and examined for CO 2 RR toward HCOOH formation. In contrast to SnO 2 nanoparticles (NPs) with a larger electrochemically active surface area (ECSA), the ultrathin SnO 2 QWs with exposed GBs show enhanced current density (j), an improved Faradaic efficiency (FE) of over 80 % for HCOOH and ca. 90 % for C1 products as well as energy efficiency (EE) of over 50 % in a wide potential window; maximum values of FE (87.3 %) and EE (52.7 %) are achieved.
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Cites
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
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Self-citationGarg, S., Li, M., Weber, A. Z., Ge, L., Li, L., Rudolph, V., Wang, G., & Rufford, T. E. (2020) · Journal of Materials Chemistry A · doi:10.1039/c9ta13298h · Cited by 478
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Metadata
- Authors
- Liu, S., Xiao, J., Lu, X. F., Wang, J., Wang, X., & Lou, X. W. (.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-05-17
- Volume
- 58
- Issue
- 25
- Pages
- 8499-8503
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2935876896
- Cited by
- 420
- References
- 34
- FWCI
- 12.83
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Liu, S., Xiao, J., Lu, X. F., Wang, J., Wang, X., & Lou, X. W. (. (2019). Efficient Electrochemical Reduction of CO2 to HCOOH over Sub‐2 nm SnO2 Quantum Wires with Exposed Grain Boundaries. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201903613
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