The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
Promoting Subordinate, Efficient Ruthenium Sites with Interstitial Silicon for Pt‐Like Electrocatalytic Activity
Abstract
The fundamental understanding and rational manipulation of catalytic site preference at extended solid surfaces is crucial in the search for advanced catalysts. Herein we find that the Ru top sites at metallic ruthenium surface have efficient Pt‐like activity for the hydrogen evolution reaction (HER), but they are subordinate to their adjacent, less active Ru 3‐hollow sites due to the stronger hydrogen‐binding ability of the latter. We also present an interstitial incorporation strategy for the promotion of the Ru top sites from subordinate to dominant character, while maintaining Pt‐like catalytic activity. Our combined theoretical and experimental studies further identify intermetallic RuSi as a highly active, non‐Pt material for catalyzing the HER, because of its suitable electronic structure governed by a good balance of ligand and strain effects.
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Cites
Noble metal-free hydrogen evolution catalysts for water splitting
Zou, X., & Zhang, Y. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00448e · Cited by 5,955
Self-citationBiomimetic Hydrogen Evolution: MoS 2 Nanoparticles as Catalyst for Hydrogen Evolution
Hinnemann, B., Moses, P. G., Bonde, J., Jørgensen, K. P., Nielsen, J. H., Horch, S., Chorkendorff, I., & Nørskov, J. K. (2005) · Journal of the American Chemical Society · doi:10.1021/ja0504690 · Cited by 4,065
An efficient and pH-universal ruthenium-based catalyst for the hydrogen evolution reaction
Mahmood, J., Li, F., Jung, S.-M., Okyay, M. S., Ahmad, I., Kim, S.-J., Park, N., Jeong, H. Y., & Baek, J.-B. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2016.304 · Cited by 1,685
Skúlason, E., Tripkovic, V., Björketun, M. E., Gudmundsdóttir, S., Karlberg, G., Rossmeisl, J., Bligaard, T., Jónsson, H., & Nørskov, J. K. (2010) · The Journal of Physical Chemistry C · doi:10.1021/jp1048887 · Cited by 1,271
Sheng, W., Myint, M., Chen, J. G., & Yan, Y. (2013) · Energy & Environmental Science · doi:10.1039/c3ee00045a · Cited by 1,202
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Self-citationWang, Z., Sun, K., Henzie, J., Hao, X., Li, C., Takei, T., Kang, Y., & Yamauchi, Y. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201801467 · Cited by 166
Cited by
Single-atom catalysts for photocatalytic energy conversion
Xue, Z.-H., Luan, D., Zhang, H., & (David) Lou, X. W. (2022) · Joule · doi:10.1016/j.joule.2021.12.011 · Cited by 567
Feng, G., Ning, F., Song, J., Shang, H., Zhang, K., Ding, Z., Gao, P., Chu, W., & Xia, D. (2021) · Journal of the American Chemical Society · doi:10.1021/jacs.1c07643 · Cited by 560
Wu, Y., Li, X., Wei, Y., Fu, Z., Wei, W., Wu, X., Zhu, Q., & Xu, Q. (2021) · Advanced Materials · doi:10.1002/adma.202006965 · Cited by 378
Li, G., Jang, H., Liu, S., Li, Z., Kim, M. G., Qin, Q., Liu, X., & Cho, J. (2022) · Nature Communications · doi:10.1038/s41467-022-28947-9 · Cited by 336
He, Q., Zhou, Y., Shou, H., Wang, X., Zhang, P., Xu, W., Qiao, S., Wu, C., Liu, H., Liu, D., et al. (2022) · Advanced Materials · doi:10.1002/adma.202110604 · Cited by 322
Metadata
- Authors
- Chen, H., Ai, X., Liu, W., Xie, Z., Feng, W., Chen, W., & Zou, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-07-03
- Volume
- 58
- Issue
- 33
- Pages
- 11409-11413
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2951262017
- Cited by
- 180
- References
- 7
- FWCI
- 5.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, H., Ai, X., Liu, W., Xie, Z., Feng, W., Chen, W., & Zou, X. (2019). Promoting Subordinate, Efficient Ruthenium Sites with Interstitial Silicon for Pt‐Like Electrocatalytic Activity. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201906394
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