The DOI matches its Crossref record; 38 of the 38 references it cites were found in a registry or an index.
Bi2O3 Nanosheets Grown on Multi‐Channel Carbon Matrix to Catalyze Efficient CO2 Electroreduction to HCOOH
Abstract
Bi 2 O 3 nanosheets were grown on a conductive multiple channel carbon matrix (MCCM) for CO 2 RR. The obtained electrocatalyst shows a desirable partial current density of ca. 17.7 mA cm−2 at a moderate overpotential, and it is highly selective towards HCOOH formation with Faradaic efficiency approaching 90 % in a wide potential window and its maximum value of 93.8 % at −1.256 V. It also exhibits a maximum energy efficiency of 55.3 % at an overpotential of 0.846 V and long‐term stability of 12 h with negligible degradation. The superior performance is attributed to the synergistic contribution of the interwoven MCCM and the hierarchical Bi 2 O 3 nanosheets, where the MCCM provides an accelerated electron transfer, increased CO 2 adsorption, and a high ratio of pyrrolic‐N and pyridinic‐N, while ultrathin Bi 2 O 3 nanosheets offer abundant active sites, lowered contact resistance and work function as well as a shortened diffusion pathway for electrolyte.
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Cites
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
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Particle Size Effects in the Catalytic Electroreduction of CO2 on Cu Nanoparticles
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Size-Dependent Electrocatalytic Reduction of CO2 over Pd Nanoparticles
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Nanostructured transition metal dichalcogenide electrocatalysts for CO 2 reduction in ionic liquid
Asadi, M., Kim, K., Liu, C., Addepalli, A. V., Abbasi, P., Yasaei, P., Phillips, P., Behranginia, A., Cerrato, J. M., Haasch, R., et al. (2016) · Science · doi:10.1126/science.aaf4767 · Cited by 907
Selective increase in CO 2 electroreduction activity at grain-boundary surface terminations
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Shape-Dependent Electrocatalytic Reduction of CO2 to CO on Triangular Silver Nanoplates
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Self-citationGrain-Boundary-Dependent CO 2 Electroreduction Activity
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
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Self-citationBismuthene for highly efficient carbon dioxide electroreduction reaction
Yang, F., Elnabawy, A. O., Schimmenti, R., Song, P., Wang, J., Peng, Z., Yao, S., Deng, R., Song, S., Lin, Y., et al. (2020) · Nature Communications · doi:10.1038/s41467-020-14914-9 · Cited by 508
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Metadata
- Authors
- Liu, S., Lu, X. F., Xiao, J., Wang, X., & Lou, X. W. (.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-08-16
- Volume
- 58
- Issue
- 39
- Pages
- 13828-13833
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2965174703
- Cited by
- 357
- References
- 38
- FWCI
- 9.89
- Type
- journal article
- Language
- en
- Open access
- closed
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