The DOI matches its Crossref record; 38 of the 38 references it cites were found in a registry or an index.
Metal–Organic Framework‐Derived Carbon Nanorods Encapsulating Bismuth Oxides for Rapid and Selective CO2 Electroreduction to Formate
Abstract
Carbon dioxide (CO 2) conversion is promising in alleviating the excessive CO 2 level and simultaneously producing valuables. This work reports the preparation of carbon nanorods encapsulated bismuth oxides for the efficient CO 2 electroconversion toward formate production. This resultant catalyst exhibits a small onset potential of −0.28 V vs. RHE and partial current density of over 200 mA cm−2 with a stable and high Faradaic efficiency of 93 % for formate generation in a flow cell configuration. Electrochemical results demonstrate the synergistic effect in the Bi 2 O 3@C promotes the rapid and selective CO 2 reduction in which the Bi 2 O 3 is beneficial for improving the reaction kinetics and formate selectivity, while the carbon matrix would be helpful for enhancing the activity and current density of formate production. This work provides effective bismuth‐based MOF derivatives for efficient formate production and offers insights in promoting practical CO 2 conversion technology.
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Cites
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Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
Lu, X. F., Fang, Y., Luan, D., & Lou, X. W. D. (2021) · Nano Letters · doi:10.1021/acs.nanolett.0c04898 · Cited by 555
Wu, Z., Wu, H., Cai, W., Wen, Z., Jia, B., Wang, L., Jin, W., & Ma, T. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202102832 · Cited by 354
Metadata
- Authors
- Deng, P., Yang, F., Wang, Z., Chen, S., Zhou, Y., Zaman, S., & Xia, B. Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-04-28
- Volume
- 59
- Issue
- 27
- Pages
- 10807-10813
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3013265070
- Cited by
- 394
- References
- 38
- FWCI
- 11.61
- Type
- journal article
- Language
- en
- Open access
- closed
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- Deng, P., Yang, F., Wang, Z., Chen, S., Zhou, Y., Zaman, S., & Xia, B. Y. (2020). Metal–Organic Framework‐Derived Carbon Nanorods Encapsulating Bismuth Oxides for Rapid and Selective CO2 Electroreduction to Formate. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202000657
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