The DOI matches its Crossref record; 9 of the 9 references it cites were found in a registry or an index.
Selective CO2 Electroreduction to Ethylene and Multicarbon Alcohols via Electrolyte‐Driven Nanostructuring
Open accessAbstract
Production of multicarbon products (C 2+) from CO 2 electroreduction reaction (CO 2 RR) is highly desirable for storing renewable energy and reducing carbon emission. The electrochemical synthesis of CO 2 RR catalysts that are highly selective for C 2+ products via electrolyte‐driven nanostructuring is presented. Nanostructured Cu catalysts synthesized in the presence of specific anions selectively convert CO 2 into ethylene and multicarbon alcohols in aqueous 0.1 m KHCO 3 solution, with the iodine‐modified catalyst displaying the highest Faradaic efficiency of 80 % and a partial geometric current density of ca. 31.2 mA cm−2 for C 2+ products at −0.9 V vs. RHE. Operando X‐ray absorption spectroscopy and quasi in situ X‐ray photoelectron spectroscopy measurements revealed that the high C 2+ selectivity of these nanostructured Cu catalysts can be attributed to the highly roughened surface morphology induced by the synthesis, presence of subsurface oxygen and Cu+ species, and the adsorbed halides.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Highly selective plasma-activated copper catalysts for carbon dioxide reduction to ethylene
Mistry, H., Varela, A. S., Bonifacio, C. S., Zegkinoglou, I., Sinev, I., Choi, Y.-W., Kisslinger, K., Stach, E. A., Yang, J. C., Strasser, P., et al. (2016) · Nature Communications · doi:10.1038/ncomms12123 · Cited by 1,214
Self-citationDopant-induced electron localization drives CO2 reduction to C2 hydrocarbons
Zhou, Y., Che, F., Liu, M., Zou, C., Liang, Z., De Luna, P., Yuan, H., Li, J., Wang, Z., Xie, H., et al. (2018) · Nature Chemistry · doi:10.1038/s41557-018-0092-x · Cited by 1,171
De Luna, P., Quintero-Bermudez, R., Dinh, C.-T., Ross, M. B., Bushuyev, O. S., Todorović, P., Regier, T., Kelley, S. O., Yang, P., & Sargent, E. H. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0018-9 · Cited by 1,046
Probing the Active Surface Sites for CO Reduction on Oxide-Derived Copper Electrocatalysts
Verdaguer-Casadevall, A., Li, C. W., Johansson, T. P., Scott, S. B., McKeown, J. T., Kumar, M., Stephens, I. E. L., Kanan, M. W., & Chorkendorff, I. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b06227 · Cited by 645
Subsurface Oxygen in Oxide-Derived Copper Electrocatalysts for Carbon Dioxide Reduction
Eilert, A., Cavalca, F., Roberts, F. S., Osterwalder, J., Liu, C., Favaro, M., Crumlin, E. J., Ogasawara, H., Friebel, D., Pettersson, L. G. M., et al. (2017) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.6b02273 · Cited by 443
Lee, S., Kim, D., & Lee, J. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201505730 · Cited by 320
Cavalca, F., Ferragut, R., Aghion, S., Eilert, A., Diaz-Morales, O., Liu, C., Koh, A. L., Hansen, T. W., Pettersson, L. G. M., & Nilsson, A. (2017) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.7b08278 · Cited by 123
Stability and Effects of Subsurface Oxygen in Oxide-Derived Cu Catalyst for CO 2 Reduction
Liu, C., Lourenço, M. P., Hedström, S., Cavalca, F., Diaz-Morales, O., Duarte, H. A., Nilsson, A., & Pettersson, L. G. M. (2017) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.7b08269 · Cited by 112
Cited by
Ma, W., Xie, S., Liu, T., Fan, Q., Ye, J., Sun, F., Jiang, Z., Zhang, Q., Cheng, J., & Wang, Y. (2020) · Nature Catalysis · doi:10.1038/s41929-020-0450-0 · Cited by 1,468
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
In Situ/Operando Electrocatalyst Characterization by X-ray Absorption Spectroscopy
Timoshenko, J., & Roldan Cuenya, B. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00396 · Cited by 931
Self-citationElectrochemical CO2 reduction (CO2RR) to multi-carbon products over copper-based catalysts
Woldu, A. R., Huang, Z., Zhao, P., Hu, L., & Astruc, D. (2022) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2021.214340 · Cited by 578
Lee, S. Y., Jung, H., Kim, N.-K., Oh, H.-S., Min, B. K., & Hwang, Y. J. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b02173 · Cited by 558
Metadata
- Authors
- Gao, D., Sinev, I., Scholten, F., Arán‐Ais, R. M., Divins, N. J., Kvashnina, K., Timoshenko, J., & Roldan Cuenya, B.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-10-08
- Volume
- 58
- Issue
- 47
- Pages
- 17047-17053
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2971788951
- Cited by
- 261
- References
- 9
- FWCI
- 6.34
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Gao, D., Sinev, I., Scholten, F., Arán‐Ais, R. M., Divins, N. J., Kvashnina, K., Timoshenko, J., & Roldan Cuenya, B. (2019). Selective CO2 Electroreduction to Ethylene and Multicarbon Alcohols via Electrolyte‐Driven Nanostructuring. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201910155
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