Fluorescence Self‐Reporting Precipitation Polymerization Based on Aggregation‐Induced Emission for Constructing Optical Nanoagents
Abstract
Precipitation polymerization is becoming increasingly popular in energy, environment and biomedicine. However, its proficient utilization highly relies on the mechanistic understanding of polymerization process. Now, a fluorescence self‐reporting method based on aggregation‐induced emission (AIE) is used to shed light on the mechanism of precipitation polymerization. The nucleation and growth processes during the copolymerization of a vinyl‐modified AIEgen, styrene, and maleic anhydride can be sensitively monitored in real time. The phase‐separation and dynamic hardening processes can be clearly discerned by tracking fluorescence changes. Moreover, polymeric fluorescent particles (PFPs) with uniform and tunable sizes can be obtained in a self‐stabilized manner. These PFPs exhibit biolabeling and photosensitizing abilities and are used as superior optical nanoagents for photo‐controllable immunotherapy, indicative of their great potential in biomedical applications.
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Self-citation
- Authors
- Wang, G., Zhou, L., Zhang, P., Zhao, E., Zhou, L., Chen, D., Sun, J., Gu, X., Yang, W., & Tang, B. Z.
- Affiliations
- State Key Laboratory of Chemical Resource Engineering (CN)
- Chinese Academy of Sciences (CN)
- Dongguan University of Technology (CN)
- Hong Kong University of Science and Technology (HK)
- Corresponding author
- Gu, Xinggui
- ORCID
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-01-09
- Volume
- 59
- Issue
- 25
- Pages
- 10122-10128
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2994810924
- Cited by
- 70
- References
- 58
- Citations by year
- 2026: 5 · 2025: 8 · 2024: 9 · 2023: 11 · 2022: 11 · 2021: 16 · 2020: 10
- FWCI
- 3.34
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Angewandte Chemie International Edition (publishedVersion)
- PubMed (publishedVersion)
- Rare & Special e-Zone (The Hong Kong University of Science and Technology) (submittedVersion)
- Funders
- National Natural Science Foundation of China (21702016)
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › Luminescence and Fluorescent Materials
- Physical Sciences › Chemistry › Organic Chemistry › Advanced Polymer Synthesis and Characterization
- Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
- Keywords
- precipitation polymerization, aggregation-induced emission, styrene, maleic anhydride, nucleation and growth, phase separation, dynamic hardening, biolabeling, photosensitization
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