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Enhanced CO2 Electroreduction on Neighboring Zn/Co Monomers by Electronic Effect
Abstract
It is of great significance to reveal the detailed mechanism of neighboring effects between monomers, as they could not only affect the intermediate bonding but also change the reaction pathway. This paper describes the electronic effect between neighboring Zn/Co monomers effectively promoting CO 2 electroreduction to CO. Zn and Co atoms coordinated on N doped carbon (ZnCoNC) show a CO faradaic efficiency of 93.2 % at −0.5 V versus RHE during a 30‐hours test. Extended X‐ray absorption fine structure measurements (EXAFS) indicated no direct metal–metal bonding and X‐ray absorption near‐edge structure (XANES) showed the electronic effect between Zn/Co monomers. In situ attenuated total reflection‐infrared spectroscopy (ATR‐IR) and density functional theory (DFT) calculations further revealed that the electronic effect between Zn/Co enhanced the *COOH intermediate bonding on Zn sites and thus promoted CO production. This work could act as a promising way to reveal the mechanism of neighboring monomers and to influence catalysis.
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Cites
Platinum single-atom and cluster catalysis of the hydrogen evolution reaction
Cheng, N., Stambula, S., Wang, D., Banis, M. N., Liu, J., Riese, A., Xiao, B., Li, R., Sham, T.-K., Liu, L.-M., et al. (2016) · Nature Communications · doi:10.1038/ncomms13638 · Cited by 2,072
Fei, H., Dong, J., Feng, Y., Allen, C. S., Wan, C., Volosskiy, B., Li, M., Zhao, Z., Wang, Y., Sun, H., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0008-y · Cited by 1,973
Self-citationPartially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
High performance platinum single atom electrocatalyst for oxygen reduction reaction
Liu, J., Jiao, M., Lu, L., Barkholtz, H. M., Li, Y., Wang, Y., Jiang, L., Wu, Z., Liu, D.-J., Zhuang, L., et al. (2017) · Nature Communications · doi:10.1038/ncomms15938 · Cited by 772
Cited by
Emerging Dual‐Atomic‐Site Catalysts for Efficient Energy Catalysis
Zhang, W., Chao, Y., Zhang, W., Zhou, J., Lv, F., Wang, K., Lin, F., Luo, H., Li, J., Tong, M., et al. (2021) · Advanced Materials · doi:10.1002/adma.202102576 · Cited by 528
Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination
Lu, B., Liu, Q., & Chen, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01950 · Cited by 394
Metadata
- Authors
- Zhu, W., Zhang, L., Liu, S., Li, A., Yuan, X., Hu, C., Zhang, G., Deng, W., Zang, K., Luo, J., Zhu, Y., Gu, M., Zhao, Z., & Gong, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-04-28
- Volume
- 59
- Issue
- 31
- Pages
- 12664-12668
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4253860825
- Cited by
- 242
- References
- 5
- FWCI
- 7.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhu, W., Zhang, L., Liu, S., Li, A., Yuan, X., Hu, C., Zhang, G., Deng, W., Zang, K., Luo, J., Zhu, Y., Gu, M., Zhao, Z., & Gong, J. (2020). Enhanced CO2 Electroreduction on Neighboring Zn/Co Monomers by Electronic Effect. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201916218
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