The DOI matches its Crossref record; 33 of the 33 references it cites were found in a registry or an index.
High‐Efficiency Oxygen Reduction to Hydrogen Peroxide Catalyzed by Nickel Single‐Atom Catalysts with Tetradentate N2O2 Coordination in a Three‐Phase Flow Cell
Abstract
Carbon‐supported Ni II single‐atom catalysts with a tetradentate Ni‐N 2 O 2 coordination formed by a Schiff base ligand‐mediated pyrolysis strategy are presented. A Ni II complex of the Schiff base ligand (R,R)‐(−)‐N,N′‐bis(3,5‐di‐tert‐butylsalicylidene)‐1,2‐cyclohexanediamine was adsorbed onto a carbon black support, followed by pyrolysis of the modified carbon material at 300 °C in Ar. The Ni‐N 2 O 2/C catalyst showed excellent performance for the electrocatalytic reduction of O 2 to H 2 O 2 through a two‐electron transfer process in alkaline conditions, with a H 2 O 2 selectivity of 96 %. At a current density of 70 mA cm−2, a H 2 O 2 production rate of 5.9 mol g cat.−1 h−1 was achieved using a three‐phase flow cell, with good catalyst stability maintained over 8 h of testing. The Ni‐N 2 O 2/C catalyst could electrocatalytically reduce O 2 in air to H 2 O 2 at a high current density, still affording a high H 2 O 2 selectivity (>90 %). A precise Ni‐N 2 O 2 coordination was key to the performance.
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Cites
Heterogeneous single-atom catalysis
Wang, A., Li, J., & Zhang, T. (2018) · Nature Reviews Chemistry · doi:10.1038/s41570-018-0010-1 · Cited by 4,191
Self-citationHydrogen Peroxide Synthesis: An Outlook beyond the Anthraquinone Process
Campos‐Martin, J. M., Blanco‐Brieva, G., & Fierro, J. L. G. (2006) · Angewandte Chemie International Edition · doi:10.1002/anie.200503779 · Cited by 3,238
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Self-citationChen, Y., Ji, S., Wang, Y., Dong, J., Chen, W., Li, Z., Shen, R., Zheng, L., Zhuang, Z., Wang, D., et al. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201702473 · Cited by 1,988
Self-citationFei, H., Dong, J., Feng, Y., Allen, C. S., Wan, C., Volosskiy, B., Li, M., Zhao, Z., Wang, Y., Sun, H., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0008-y · Cited by 1,973
Self-citationZhao, C., Dai, X., Yao, T., Chen, W., Wang, X., Wang, J., Yang, J., Wei, S., Wu, Y., & Li, Y. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b02736 · Cited by 1,365
Atomic-level tuning of Co–N–C catalyst for high-performance electrochemical H2O2 production
Jung, E., Shin, H., Lee, B.-H., Efremov, V., Lee, S., Lee, H. S., Kim, J., Hooch Antink, W., Park, S., Lee, K.-S., et al. (2020) · Nature Materials · doi:10.1038/s41563-019-0571-5 · Cited by 1,247
Toward the Decentralized Electrochemical Production of H2O2: A Focus on the Catalysis
Yang, S., Verdaguer-Casadevall, A., Arnarson, L., Silvioli, L., Čolić, V., Frydendal, R., Rossmeisl, J., Chorkendorff, I., & Stephens, I. E. L. (2018) · ACS Catalysis · doi:10.1021/acscatal.8b00217 · Cited by 1,215
Electrochemical synthesis of hydrogen peroxide from water and oxygen
Perry, S. C., Pangotra, D., Vieira, L., Csepei, L.-I., Sieber, V., Wang, L., Ponce de León, C., & Walsh, F. C. (2019) · Nature Reviews Chemistry · doi:10.1038/s41570-019-0110-6 · Cited by 1,133
Single‐Atom Catalysts: Emerging Multifunctional Materials in Heterogeneous Catalysis
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Cited by
Cation‐Vacancy‐Enriched Nickel Phosphide for Efficient Electrosynthesis of Hydrogen Peroxides
Zhou, Z., Kong, Y., Tan, H., Huang, Q., Wang, C., Pei, Z., Wang, H., Liu, Y., Wang, Y., Li, S., et al. (2022) · Advanced Materials · doi:10.1002/adma.202106541 · Cited by 325
Self-citationZhao, S., Li, J., Wang, R., Cai, J., & Zang, S. (2022) · Advanced Materials · doi:10.1002/adma.202107291 · Cited by 270
Zhao, Q., Wang, Y., Lai, W.-H., Xiao, F., Lyu, Y., Liao, C., & Shao, M. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00878a · Cited by 269
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Metadata
- Authors
- Wang, Y., Shi, R., Shang, L., Waterhouse, G. I. N., Zhao, J., Zhang, Q., Gu, L., & Zhang, T.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-05-25
- Volume
- 59
- Issue
- 31
- Pages
- 13057-13062
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3020718800
- Cited by
- 384
- References
- 33
- FWCI
- 10.12
- Type
- journal article
- Language
- en
- Open access
- closed
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