Enhancing Li+ Transport in NMC811||Graphite Lithium‐Ion Batteries at Low Temperatures by Using Low‐Polarity‐Solvent Electrolytes
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LiNixCoyMnzO 2 (x+y+z=1)||graphite lithium‐ion battery (LIB) chemistry promises practical applications. However, its low‐temperature (≤ −20 °C) performance is poor because the increased resistance encountered by Li+ transport in and across the bulk electrolytes and the electrolyte/electrode interphases induces capacity loss and battery failures. Though tremendous efforts have been made, there is still no effective way to reduce the charge transfer resistance (Rct) which dominates low‐temperature LIBs performance. Herein, we propose a strategy of using low‐polarity‐solvent electrolytes which have weak interactions between the solvents and the Li+ to reduce Rct, achieving facile Li+ transport at sub‐zero temperatures. The exemplary electrolyte enables LiNi 0.8 Mn 0.1 Co 0.1 O 2||graphite cells to deliver a capacity of ≈113 mAh g−1 (98 % full‐cell capacity) at 25 °C and to remain 82 % of their room‐temperature capacity at −20 °C without lithium plating at 1/3C. They also retain 84 % of their capacity at −30 °C and 78 % of their capacity at −40 °C and show stable cycling at 50 °C.
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Ethyl methyl carbonate has a wide liquid temperature range from -53 to 110 °C and a very small dipole moment, which enhances kinetics and reduces charge transfer resistance for the desolvation process.
“EMC has a wide liquid temperature range from -53 to 110 °C with a very small dipole moment, which enhances the kinetics and reduces the charge transfer resistance for the desolvation process.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [29]
A graphite-NMC811 pouch cell using the 2.0 M LiFSI in EMC:TTE electrolyte showed enhanced cyclic stability across a wide temperature range from -40 to 50 °C.
“As a result, the graphite-NMC811 pouch cell showed enhanced cyclic stability operating across a wide-temperature range from -40 to 50 °C.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [29]
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A High-voltage and Low-solvating Electrolyte Towards Promising Micro-Si/Ni-rich NMC Full Cells
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“To further reduce interfacial resistance and enhance desolvation kinetics, Nan et al. [ 121 ] selected a low-polarity solvent (EMC, dipole moment: 0.89 D) together with the diluent TTE to construct a WSE (DE: 2 M LiFSI-EMC/TTE).”
InfluentialSelf-citation
- Authors
- Nan, B., Chen, L., Rodrigo, N. D., Borodin, O., Piao, N., Xia, J., Pollard, T., Hou, S., Zhang, J., Ji, X., Xu, J., Zhang, X., Ma, L., He, X., Liu, S., Wan, H., Hu, E., Zhang, W., Xu, K., Yang, X., Lucht, B., & Wang, C.
- Affiliations
- University of Maryland, College Park (US)
- University of Rhode Island (US)
- DEVCOM Army Research Laboratory (US)
- Department of Chemical and Biomolecular Engineering University of Maryland College Park MD 20742 USA
- University of North Carolina at Charlotte (US)
- Brookhaven National Laboratory (US)
- Corresponding author
- Wang, Chunsheng
- ORCID
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-07-20
- Volume
- 61
- Issue
- 35
- Pages
- e202205967-e202205967
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4283823340
- Cited by
- 222
- References
- 51
- Citations by year
- 2026: 35 · 2025: 58 · 2024: 73 · 2023: 50 · 2022: 6
- FWCI
- 12.79
- Type
- journal article
- Language
- en
- Open access
- Locations
- Angewandte Chemie International Edition (publishedVersion)
- PubMed (publishedVersion)
- Journal of Media Literacy Education (submittedVersion, cc-by)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
- Keywords
- NMC811, lithium-ion batteries, low-temperature performance, Li+ transport, charge transfer resistance, LiNi0.8Co0.1Mn0.1O2, graphite anode, lithium plating, capacity retention
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