Cited by 222Advancements in Battery MaterialsAdvanced Battery Materials and TechnologiesBattery Modeling and Management

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Enhancing Li+ Transport in NMC811||Graphite Lithium‐Ion Batteries at Low Temperatures by Using Low‐Polarity‐Solvent Electrolytes

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Nan, Bo, Chen, Long, Rodrigo, Nuwanthi D., Borodin, Oleg, Piao, Nan, Xia, Jiale, Pollard, Travis, Hou, Singyuk, Zhang, Jiaxun, Ji, Xiao, Xu, Jijian, Zhang, Xiyue, Ma, Lin, He, Xinzi, Liu, Sufu, Wan, Hongli, Hu, Enyuan, Zhang, Weiran, Xu, Kang, Yang, Xiao‐Qing, Lucht, Brett, Wang, Chunsheng·2022·Angewandte Chemie International Edition

DOI 10.1002/anie.202205967

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Abstract

LiNixCoyMnzO 2 (x+y+z=1)||graphite lithium‐ion battery (LIB) chemistry promises practical applications. However, its low‐temperature (≤ −20 °C) performance is poor because the increased resistance encountered by Li+ transport in and across the bulk electrolytes and the electrolyte/electrode interphases induces capacity loss and battery failures. Though tremendous efforts have been made, there is still no effective way to reduce the charge transfer resistance (Rct) which dominates low‐temperature LIBs performance. Herein, we propose a strategy of using low‐polarity‐solvent electrolytes which have weak interactions between the solvents and the Li+ to reduce Rct, achieving facile Li+ transport at sub‐zero temperatures. The exemplary electrolyte enables LiNi 0.8 Mn 0.1 Co 0.1 O 2||graphite cells to deliver a capacity of ≈113 mAh g−1 (98 % full‐cell capacity) at 25 °C and to remain 82 % of their room‐temperature capacity at −20 °C without lithium plating at 1/3C. They also retain 84 % of their capacity at −30 °C and 78 % of their capacity at −40 °C and show stable cycling at 50 °C.

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Authors: Nan, B., Chen, L., Rodrigo, N. D., Borodin, O., Piao, N., Xia, J., Pollard, T., Hou, S., Zhang, J., Ji, X., Xu, J., Zhang, X., Ma, L., He, X., Liu, S., Wan, H., Hu, E., Zhang, W., Xu, K., Yang, X., Lucht, B., & Wang, C.
Affiliations: University of Maryland, College Park (US)
University of Rhode Island (US)
DEVCOM Army Research Laboratory (US)
Department of Chemical and Biomolecular Engineering University of Maryland College Park MD 20742 USA
University of North Carolina at Charlotte (US)
Brookhaven National Laboratory (US)
Corresponding author: Wang, Chunsheng
ORCID: Nan, Bo
Chen, Long
Rodrigo, Nuwanthi D.
Borodin, Oleg
Piao, Nan
Xia, Jiale
Pollard, Travis
Hou, Singyuk
Zhang, Jiaxun
Ji, Xiao
Zhang, Xiyue
He, Xinzi
Liu, Sufu
Hu, Enyuan
Xu, Kang
Lucht, Brett
Wang, Chunsheng
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2022-07-20
Volume: 61
Issue: 35
Pages: e202205967-e202205967
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.202205967
OpenAlex: W4283823340
Cited by: 222
References: 51
Citations by year: 2026: 35 · 2025: 58 · 2024: 73 · 2023: 50 · 2022: 6
FWCI: 12.79
Type: journal article
Language: en
Open access: green
digitalcommons.uri.edu
Licence: cc-by
onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
Journal of Media Literacy Education (submittedVersion, cc-by)
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
Physical Sciences › Engineering › Automotive Engineering › Battery Modeling and Management
Keywords: NMC811, lithium-ion batteries, low-temperature performance, Li+ transport, charge transfer resistance, LiNi0.8Co0.1Mn0.1O2, graphite anode, lithium plating, capacity retention

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Enhancing Li+ Transport in NMC811||Graphite Lithium‐Ion Batteries at Low Temperatures by Using Low‐Polarity‐Solvent Electrolytes

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