The DOI matches its Crossref record; 52 of the 52 references it cites were found in a registry or an index.
P and Cu Dual Sites on Graphitic Carbon Nitride for Photocatalytic CO2Reduction to Hydrocarbon Fuels with High C2H6Evolution
Abstract
The light‐driven CO 2 reduction to multi‐carbon products is especially meaningful, while the low efficiency of multi‐electron transfer and sluggish C−C coupling greatly hinder its development. Herein, we report a photocatalyst comprising of P and Cu dual sites anchored on graphitic carbon nitride (P/Cu SAs@CN), which achieves a high C 2 H 6 evolution rate of 616.6 μmol g−1 h−1 in reducing CO 2 to hydrocarbons. The detailed spectroscopic characterizations identify the formation of charge‐enriched Cu sites, where the isolated P atoms serve as hole capture sites during photocatalysis. Theoretical simulations combined with in situ FTIR measurement reveal a kinetically feasible process for the formation of C−C coupling intermediate (*OC−COH) and confirm the favorable production of C 2 H 6 on the P/Cu SAs@CN photocatalyst. This work offers new insights into the photocatalyst design with atomic precision toward highly efficient photocatalytic CO 2 conversion to high value‐added carbon products.
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Cites
Photocatalytic Reduction of CO2 on TiO2 and Other Semiconductors
Habisreutinger, S. N., Schmidt‐Mende, L., & Stolarczyk, J. K. (2013) · Angewandte Chemie International Edition · doi:10.1002/anie.201207199 · Cited by 2,989
Titanium Dioxide-Based Nanomaterials for Photocatalytic Fuel Generations
Ma, Y., Wang, X., Jia, Y., Chen, X., Han, H., & Li, C. (2014) · Chemical Reviews · doi:10.1021/cr500008u · Cited by 2,411
Li, X., Sun, Y., Xu, J., Shao, Y., Wu, J., Xu, X., Pan, Y., Ju, H., Zhu, J., & Xie, Y. (2019) · Nature Energy · doi:10.1038/s41560-019-0431-1 · Cited by 1,636
Hierarchical Porous O‐Doped g‐C3N4 with Enhanced Photocatalytic CO2 Reduction Activity
Fu, J., Zhu, B., Jiang, C., Cheng, B., You, W., & Yu, J. (2017) · Small · doi:10.1002/smll.201603938 · Cited by 1,291
Teng, Z., Zhang, Q., Yang, H., Kato, K., Yang, W., Lu, Y.-R., Liu, S., Wang, C., Yamakata, A., Su, C., et al. (2021) · Nature Catalysis · doi:10.1038/s41929-021-00605-1 · Cited by 1,113
A Hierarchical Z‑Scheme α‐Fe2O3/g‐C3N4 Hybrid for Enhanced Photocatalytic CO2 Reduction
Jiang, Z., Wan, W., Li, H., Yuan, S., Zhao, H., & Wong, P. K. (2018) · Advanced Materials · doi:10.1002/adma.201706108 · Cited by 948
Theoretical Considerations on the Electroreduction of CO to C 2 Species on Cu(100) Electrodes
Calle‐Vallejo, F., & Koper, M. T. M. (2013) · Angewandte Chemie International Edition · doi:10.1002/anie.201301470 · Cited by 941
Molecular electrocatalysts can mediate fast, selective CO 2 reduction in a flow cell
Ren, S., Joulié, D., Salvatore, D., Torbensen, K., Wang, M., Robert, M., & Berlinguette, C. P. (2019) · Science · doi:10.1126/science.aax4608 · Cited by 941
CO2 Reduction: From the Electrochemical to Photochemical Approach
Wu, J., Huang, Y., Ye, W., & Li, Y. (2017) · Advanced Science · doi:10.1002/advs.201700194 · Cited by 937
Photocatalytic CO 2 Reduction to C2+ Products
Albero, J., Peng, Y., & García, H. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c00478 · Cited by 899
Cited by
Microenvironment Engineering of Single/Dual‐Atom Catalysts for Electrocatalytic Application
Gao, Y., Liu, B., & Wang, D. (2023) · Advanced Materials · doi:10.1002/adma.202209654 · Cited by 319
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Metadata
- Authors
- Wang, G., Chen, Z., Wang, T., Wang, D., & Mao, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-08-29
- Volume
- 61
- Issue
- 40
- Pages
- e202210789-e202210789
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4291795553
- Cited by
- 312
- References
- 52
- FWCI
- 11.96
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, G., Chen, Z., Wang, T., Wang, D., & Mao, J. (2022). P and Cu Dual Sites on Graphitic Carbon Nitride for Photocatalytic CO2Reduction to Hydrocarbon Fuels with High C2H6Evolution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202210789
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