The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Cation−Solvent, Cation−Anion, and Solvent−Solvent Interactions with Electrolyte Solvation in Lithium Batteries
Abstract
Electrolyte solvation is a fundamental issue that regulates the lithium (Li) ion solvation sheath structure, the formation of cathode/anode−electrolyte interphase, and the plating/stripping behavior of Li ions in working Li batteries. Herein, we probe the cation‐solvent, cation‐anion, and solvent‐solvent interactions under both vacuum and electrolyte conditions through density functional theory calculations. The solvation effects can significantly weaken the aforementioned interactions in electrolytes as well as increase the Li−O/F distances in Li+‐containing complexes. The dissolution behaviour of Li salts in electrolytes was further explored and experimentally validated by dissolving lithium nitrate in different solvents. This work affords a mechanistic understanding of electrolyte microstructure and highlights the significant role of electrolyte solvation in regulating battery performance, affording fruitful insights into emerging electrolyte design for high‐performance batteries.
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Citations
Cites
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Cited by
Regulating Interfacial Chemistry in Lithium‐Ion Batteries by a Weakly Solvating Electrolyte**
Yao, Y., Chen, X., Yan, C., Zhang, X., Cai, W., Huang, J., & Zhang, Q. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202011482 · Cited by 855
Self-citationEmerging Chemistry for Wide-Temperature Sodium-Ion Batteries
Zhang, F., He, B., Xin, Y., Zhu, T., Zhang, Y., Wang, S., Li, W., Yang, Y., & Tian, H. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00728 · Cited by 357
Holoubek, J., Yu, M., Yu, S., Li, M., Wu, Z., Xia, D., Bhaladhare, P., Gonzalez, M. S., Pascal, T. A., Liu, P., et al. (2020) · ACS Energy Letters · doi:10.1021/acsenergylett.0c00643 · Cited by 351
Advanced energy materials for flexible batteries in energy storage: A review
Kong, L., Tang, C., Peng, H., Huang, J., & Zhang, Q. (2020) · SmartMat · doi:10.1002/smm2.1007 · Cited by 316
Self-citationWu, Y., Hu, Q., Liang, H., Wang, A., Xu, H., Wang, L., & He, X. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202300259 · Cited by 270
Metadata
- Authors
- Chen, X., Zhang, X., Li, H., & Zhang, Q.
- Venue
- Batteries & Supercaps
- Publisher
- Wiley
- Published
- 2019-01-11
- Volume
- 2
- Issue
- 2
- Pages
- 128-131
- ISSN
- 2566-6223 (ISSN-L)
- OpenAlex
- W2902278684
- Cited by
- 248
- References
- 2
- FWCI
- 5.64
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, X., Zhang, X., Li, H., & Zhang, Q. (2019). Cation−Solvent, Cation−Anion, and Solvent−Solvent Interactions with Electrolyte Solvation in Lithium Batteries. Batteries & Supercaps. https://doi.org/10.1002/batt.201800118
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